Visible light-driven oxidation of non-native substrate by laccase attached on Ru-based metal-organic frameworks

Huang, Wenguang; Zhang, Wentao; Chen, Guantongyi; Chen, Yun; Ma, Jun; Huang, Dawei; Zhao, Qinzheng; Wu, Bingdang

doi:10.1016/j.jes.2023.02.047

Cited by 3 publications

(2 citation statements)

References 86 publications

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“…Enzyme immobilisation using nanomaterials as a carrier has a racted recent a ention because of good On the other hand, the most widely used inorganic materials are hydroxyapatite [96], gold [97,98], iron oxide [99], zirconia [100], titania [101,102], silica [103][104][105][106][107], silver [108,109], zinc oxide [110], alumina [111], celite [112], and inorganic clays [113]. The most recently studied enzyme carriers include graphene-based nanomaterials [114][115][116], metalorganirameworks (MOFs) [117][118][119][120][121][122][123], and covalent organic frameworks [124][125][126][127][128][129]. The advantages of inorganic support compared with their organic counterparts are chemical, mechanical, and thermal resistance, rigidity, porosity, more reusable, and stiffness, which guarantee the stability of the novel immobilised enzyme.…”

Section: Enzyme Immobilisation Via Nanocarriersmentioning

confidence: 99%

Recent Advances in Enzyme Immobilisation Strategies: An Overview of Techniques and Composite Carriers

Mohidem,

Mohamad,

Rashid

et al. 2023

J. Compos. Sci.

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For over a century, enzyme immobilisation has been proven to be a superior strategy to improve catalytic activity and reusability and ensure easy separation, easy operation, and reduced cost. Enzyme immobilisation allows for an easier separation of the enzyme from the reaction mixture, thus simplifying downstream processing. This technology protects the enzyme from degradation or inactivation by harsh reaction conditions, making it more robust and suitable to be used in various applications. Recent strategies of immobilisation methods, such as adsorption, cross-linking, entrapment or encapsulation, and covalent bonding, were critically reviewed. These strategies have shown promising results in improving enzyme stability, activity, and reusability in various applications. A recent development in enzyme immobilisation in nanomaterials and agrowaste renewable carriers is underlined in the current review. Furthermore, the use of nanomaterials and agrowaste carriers in enzyme immobilisation has gained significant attention due to their unique properties, such as high surface area, high mass transfer, biocompatibility, and sustainability. These materials offer promising outcomes for developing more efficient and sustainable immobilised enzymes. This state-of-the-art strategy allows for better control over enzyme reactions and enhances their reusability, leading to more cost-effective and environmentally friendly processes. The use of renewable materials also helps to reduce waste generation and promote the utilisation of renewable resources, further contributing to the development of a circular economy.

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Section: Enzyme Immobilisation Via Nanocarriersmentioning

confidence: 99%

Recent Advances in Enzyme Immobilisation Strategies: An Overview of Techniques and Composite Carriers

Mohidem,

Mohamad,

Rashid

et al. 2023

J. Compos. Sci.

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“…Metal organic frameworks (MOFs) are a kind of microporous solid adsorbent material which has been widely investigated and applied in the field of materials and chemistry in recent years. MOFs are constructed from metal nodes and organic linkers [7][8][9][10][11][12][13][14]. Metal ions such as di-, tri-or tetravalent metal ions form inorganic clusters in MOFs as coordination centers.…”

Section: Introductionmentioning

confidence: 99%

One-Pot Preparation of HCPT@IRMOF-3 Nanoparticles for pH-Responsive Anticancer Drug Delivery

Cheng

2023

Molecules

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Metal–organic frameworks (MOFs) are considered to be promising materials for drug delivery. In this work, a Zinc-based MOF nanocomposite IRMOF-3 was introduced as a drug carrier for 10-hydroxycamptothecine (HCPT). Without an extra drug-loading process, a nanoscale drug delivery material HCPT@IRMOF-3 was prepared via one-pot synthesis. The composition and structure of the material were investigated, and the drug release character was measured. Compared with preparing IRMOF-3 first and loading the drug, the one-pot-prepared HCPT@IRMOF-3 exhibited a higher drug-loading capacity. The material presented pH-responsive release. The HCPT release rate at pH 5.0 was significantly higher than that at pH 7.4. The cytotoxicity experiments showed that IRMOF-3 was non-toxic, and HCPT@IRMOF-3 exhibited notable cytotoxicity to Hela and SH-SY5Y cells. One-pot synthesis is a simple and rapid method for the preparation of an MOF drug delivery system, and IRMOF-3 can be potentially used in pH-responsive drug delivery systems.

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Construction of immobilized laccase hydrogels via sodium alginate-dopamine/polyethylene glycol and its efficient degradation of dyeing wastewater

Su,

Yang,

Long

et al. 2024

International Journal of Biological Macromolecules

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Visible light-driven oxidation of non-native substrate by laccase attached on Ru-based metal-organic frameworks

Cited by 3 publications

References 86 publications

Recent Advances in Enzyme Immobilisation Strategies: An Overview of Techniques and Composite Carriers

Recent Advances in Enzyme Immobilisation Strategies: An Overview of Techniques and Composite Carriers

One-Pot Preparation of HCPT@IRMOF-3 Nanoparticles for pH-Responsive Anticancer Drug Delivery

Construction of immobilized laccase hydrogels via sodium alginate-dopamine/polyethylene glycol and its efficient degradation of dyeing wastewater

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