Abstract:Electrostatic potentials strongly affect molecular energy levels and charge states, providing the fascinating opportunity of molecular gating. Their influence on molecular vibrations remains less explored. Here, we investigate ethyl‐diaminodicyanoquinone molecules on a monolayer of MoS2 on Au(111) using scanning tunneling and atomic force microscopy and spectroscopy. These molecules exhibit a large dipole moment in gas phase, which is found to (partially) persist on the MoS2 monolayer. The self‐assembled struc… Show more
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