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doi:10.1021/cg060134

DOI: 10.1021/cg060134

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Cited by 7 publications

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Synthesis of Organized Layered Carbon by Self‐Templating of Dithiooxamide

Zhu

Yang

et al. 2016

Advanced Materials

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An unusual small molecule, dithiooxamide is used to produce nanostructured carbon via direct pyrolysis. The carbon shows a unique 2D-layer assembled structure and is in situ dual-heteroatom (N and S)-doped, meanwhile having relatively high surface area. These carbon materials can be further decorated with inorganic parts via a precomplexing approach. The functionalized carbon and the hybrid nanomaterials demonstrate remarkable performance for lithium-ion storage.

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Synthesis of Organized Layered Carbon by Self‐Templating of Dithiooxamide

Zhu

Yang

et al. 2016

Advanced Materials

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Metal‐organic frameworks for highly efficient adsorption of dibenzothiophene from liquid fuels

Tang

Huang

et al. 2016

AIChE Journal

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By taking desulfurization of liquid fuels as a demonstrative example, a bottom‐up selection was performed to find the metal‐organic frameworks (MOF)‐type adsorbents with highly efficient adsorption performance of large molecules. Through carefully analyzing the adsorption mechanism for typical S‐heterocyclic compounds like dibenzothiophene (DBT), PCN‐10 was selected in consideration of the simultaneous inclusion of several kinds of interactions in the framework. Experimental results demonstrate that this MOF exhibits extraordinary high DBT adsorption capacity (75.24 mg S g−1), showing record uptake among all the reported porous materials for the removal of thiophenicsulfur from fuels (below 1000 ppmwS), to the best of our knowledge. Moreover, the removal rate for the low sulfur concentration (50 ppmwS) can reach beyond 99%. This strategy can be conveniently extended to the screening and design of MOFs for the efficient removal of other important large guest molecules. © 2016 American Institute of Chemical Engineers AIChE J, 62: 4491–4496, 2016

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Experimental and Computational Study of Organic Sulfur Removal Proficiency of (Ni, Cu, Co)‐Doped ZIF‐8 Adsorbents

Saeedirad

Ganjali

Rashidi³

et al. 2020

ChemistrySelect

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The synthesis and characterization of a series of metal‐doped ZIF‐8 (metal=Ni, Co and Cu) has been introduced to gain the highly efficient adsorption of dibenzothiophene (DBT) in liquid phase. Under 150 ml DBT/iso‐octane, 100–1700 ppm, and 25–85 °C, the excellent efficiency and reusability in DBT removal was achieved and fitted better with the pseudo‐first order reaction. The maximum adsorption of 191.84 mg S/g for Ni/ZIF‐8 and two steps for intraparticle diffusion study contrary to Cu‐ and Co‐ZIF‐8 suggested the presence of Ni‐HMeIM clusters in ZIF‐8 cavities. Comparing the performance of prepared adsorbents, the order of qmax and PC was the same, i. e. PC Ni/ZIF‐8> PC Cu/ZIF‐8>PC Co/ZIF‐8>PC ZIF‐8 and qmax (Ni/ZIF‐8)> qmax (Cu/ZIF‐8)> qmax (Co/ZIF‐8)> qmax (ZIF‐8) for both 10% and 100% BT. The prepared adsorbents had the FoMs ranging from 0.05‐0.07 that compared to other adsorbents showed the beneficial use for large scale desulfurization process. The endothermic behavior and a homogeneous adsorption was then indicated through thermodynamic and equilibrium studies.

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Cited by 7 publications

References 0 publications

Synthesis of Organized Layered Carbon by Self‐Templating of Dithiooxamide

Synthesis of Organized Layered Carbon by Self‐Templating of Dithiooxamide

Metal‐organic frameworks for highly efficient adsorption of dibenzothiophene from liquid fuels

Experimental and Computational Study of Organic Sulfur Removal Proficiency of (Ni, Cu, Co)‐Doped ZIF‐8 Adsorbents

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