“…For the ratio between these two groups, we follow Baker (1987), who indicated that if a stem is present, about 25% of the radioactivity will be on particle surfaces and the rest will be present within the volume of particles that did not have a condensation nucleus. For the calculation of the lognormal distribution, we follow Ledger (2015) as depicted in eqn (B1): F()r=1italicβr2πe−12ln()r−αnβ2,with α defined as: αn=ln()rmean+nβ2,and where r is the particle radius, r mean is the mean particle radius, and n indicates the type of activity distribution for the particle: n = 0 for radius, n = 2 for surface, and n = 3 for volume. The parameter β is defined as ln( σ ), where σ is the standard deviation of the particle radius.…”