“…In terms of the sedimentary removal pathway, it appears that for sedimentary conditions near those for conversion of Fe 3+ to Fe 2+ , soluble U (VI) is reduced, perhaps through microbial mediation, to insoluble U (IV) (e.g., Cochran et al, 1986;Anderson, 1987;McKee et al, 1987;Barnes and Cochran, 1990;Lovley et al, 1991;Lovley et al, 1993;Fredrickson et al, 2000;King et al, 2000;Chaillou et al, 2002;Sani et al, 2004). Because this reduction potential is typically achieved in close proximity to the sediment-water boundary in continental shelf and slope environments, these sediments have elevated U concentrations relative to oxic environments (Dorta and Rona, 1971;Mo et al, 1973;Veeh et al, 1974;Degens et al, 1977;Bloch, 1980;Yamada and Tsunogai, 1983/84;Anderson et al, 1989a,b;Calvert and Pedersen, 1993;Legeleux et al, 1994;Morford and Emerson, 1999;Dunk et al, 2002;Nameroff et al, 2002;and others).…”