Unveiling the Surface Chemical Reactions during Multi-Phase Catalytic Oxidation of Soot on Nanoengineering/Interfacing/Doping-Prepared Mn-CeO2 Catalysts Using TG-MS and Operando DRIFTS-MS
Yan Sun,
Shiyu Fang,
Jiacheng Xu
et al.
Abstract:The aerosol pyrolysis method from nitrate precursors was used to prepare the Mn-CeO 2 catalyst containing Mn 2 O 3 , CeO 2 , and Mn-doped CeO 2 nanoparticles for catalyzing carbonous soot oxidation. The prepared Mn-CeO 2 catalysts have high specific surface areas, Ce 3+ ratio, and oxygen vacancy defects; these are a benefit for soot oxidation. The T 50 for soot oxidation on the 0.57Mn-CeO 2 catalyst is as low as 355 °C, which is 329 °C lower than that for soot oxidation without a catalyst. The catalysts were c… Show more
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