Abstract:Since the seminal work of Zhang
in 2016, donor-acceptor cyanoarene-based fluorophores, such as
1,2,3,5-tetrakis(carbazol-9-yl)-4,6-dicyanobenzene (4CzIPN), have been widely applied
in photoredox catalysis, and used as excellent metal-free alternatives to noble
metal Ir- and Ru-based photocatalysts. However, all the reported photoredox
reactions involving this chromophore family are based on harnessing the energy
from a single visible light photon, with a limited range of redox potentials
from -1.92 V to +1.79 … Show more
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