Unraveling Valence Electron Number Dependent Excitonic Effects over M1-N3C1 Sites in Single-Atom Catalysts
Dingren Ma,
Zhuoyun Tang,
Xinyi Guan
et al.
Abstract:Excitonic effects significantly influence the selective generation of reactive oxygen species and photothermal conversion efficiency in photocatalytic reactions; however, the intrinsic factors governing excitonic effects remain elusive. Herein, a series of single-atom catalysts with well-defined M 1 -N 3 C 1 (M = Mn, Fe, Co, and Ni) active sites are designed and synthesized to investigate the structure− activity relationship between photocatalytic materials and excitonic effects. Comprehensive characterization… Show more
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