Unlocking a Dual‐Channel Pathway in CO2 Hydrogenation to Methanol over Single‐Site Zirconium on Amorphous Silica
Meng Yang,
Jiafeng Yu,
Anna Zimina
et al.
Abstract:Converting CO2 into methanol on a large scale is of great significance in the sustainable methanol economy. Zirconia species are considered to be an essential support in Cu‐based catalysts due to their excellent properties for CO2 adsorption and activation. However, the evolution of Zr species during the reaction and the effect of their structure on the reaction pathways remain unclear. Herein, single‐site Zr species in an amorphous SiO2 matrix are created by enhancing the Zr−Si interaction in Cu/ZrO2‐SiO2 cat… Show more
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