“…Below this deconfinement temperature charge excitations lose their 1D character and resemble more and more what is expected in Fermi liquids (quasiparticles), leading in turn to a quadratic temperature dependence for the longitudinal resistivity. However, electron excitations of this "Fermi liquid" retain a low energy gap in the far infra-red spectrum in which most of the oscillator strength is carried by states above the gap coexisting with a very narrow and intense zero frequency peak in the conductivity [82,83].…”
This survey provides a brief account for the start of organic superconductivity motivated by the quest for high T c superconductors and its development since the eighties'. Besides superconductivity found in 1D organics in 1980, progresses in this field of research have contributed to better understand the physics of low dimensional conductors highlighted by the wealth of new remarkable properties. Correlations conspire to govern the low temperature properties of the metallic phase. The contribution of antiferromagnetic fluctuations to the interchain Cooper pairing proposed by the theory is borne out by experimental investigations and supports supercondutivity emerging from a non Fermi liquid background. Quasi one dimensional organic superconductors can therefore be considered as simple prototype systems for the more complex high T c materials.
“…Below this deconfinement temperature charge excitations lose their 1D character and resemble more and more what is expected in Fermi liquids (quasiparticles), leading in turn to a quadratic temperature dependence for the longitudinal resistivity. However, electron excitations of this "Fermi liquid" retain a low energy gap in the far infra-red spectrum in which most of the oscillator strength is carried by states above the gap coexisting with a very narrow and intense zero frequency peak in the conductivity [82,83].…”
This survey provides a brief account for the start of organic superconductivity motivated by the quest for high T c superconductors and its development since the eighties'. Besides superconductivity found in 1D organics in 1980, progresses in this field of research have contributed to better understand the physics of low dimensional conductors highlighted by the wealth of new remarkable properties. Correlations conspire to govern the low temperature properties of the metallic phase. The contribution of antiferromagnetic fluctuations to the interchain Cooper pairing proposed by the theory is borne out by experimental investigations and supports supercondutivity emerging from a non Fermi liquid background. Quasi one dimensional organic superconductors can therefore be considered as simple prototype systems for the more complex high T c materials.
“…However, the frequency dependence of the optical conductivity is inconsistent with a Drude-like metallic state. 33,34,23 The lowenergy peak carries only 1% of the total spectral weight and is too narrow to be interpreted as a Drude peak with a frequency-independent scattering time. It has been proposed that this peak is due to a collective mode that bears some similarities with the sliding of a charge-density wave -an interpretation supported by the new phonon features that emerge at low temperature.…”
Section: The Strong-correlation Picturementioning
confidence: 99%
“…It has been proposed that this peak is due to a collective mode that bears some similarities with the sliding of a charge-density wave -an interpretation supported by the new phonon features that emerge at low temperature. 33 Furthermore, 99% of the total spectral weight is found in a finite energy peak around 200 cm −1 . It has been suggested that this peak is a remnant of a 1 4 -filled Mott gap ∆ ρ , observed in the less metallic Fabre salts at ambient pressure.…”
Section: The Strong-correlation Picturementioning
confidence: 99%
“…24 Besides the presence of spin fluctuations at low temperature, charge fluctuations have also been observed in the normal phase via optical conductivity measurements. 33 …”
Section: The Normal Phase Above the Superconducting Phasementioning
confidence: 99%
“…2.2.). 53,54,33 Within the framework of an extended anisotropic Hubbard model, recent RPA calculations have shown that the triplet f -wave pairing can overcome the singlet d x 2 −y 2 -wave pairing when the intrachain interactions are chosen such as to boost the CDW fluctuations with respect to the SDW ones. 126,127,128 In a half-filled model, this however requires the nearest-neighbor (intrachain) interaction V to exceed U/2.…”
Section: Microscopic Theories Of the Superconducting Statementioning
We review the current understanding of superconductivity in the quasi-onedimensional organic conductors of the Bechgaard and Fabre salt families.We discuss the interplay between superconductivity, antiferromagnetism, and charge-density-wave fluctuations. The connection to recent experimental observations supporting unconventional pairing and the possibility of a tripletspin order parameter for the superconducting phase is also presented.
Infrared spectroscopy has emerged as a premier experimental technique to
probe enigmatic effects arising from strong correlations in solids. Here we
report on recent advances in this area focusing on common patterns in
correlated electron systems including transition metal oxides, intermetallics
and organic conductors. All these materials are highly conducting substances
but their electrodynamic response is profoundly different from the canonical
Drude behavior observed in simple metals. These unconventional properties can
be attributed in several cases to the formation of spin and/or charge ordered
states, zero temperature phase transitions and strong coupling to bosonic
modes
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