“…Apart from the complexity of environmental processes and interface interactions (Holnicki and Nahorski, 2015;Irwin, 2014), variance in measured and estimated pollutant concentrations where GI is present may be due to: (i) pollutant measurement error; (ii) model input uncertainties (Table 2); (iii) simplification of deposition processes (Section 3); and (iv) difficulties in treating GI in numerical solutions (Sections 4 and 5). Past studies have reported the effects of input data uncertainties on pollutant concentrations at different spatial scales, including: meteorology data uncertainty at mesoscale (Gilliam et al, 2015;Godowitch et al, 2015), emissions data uncertainty at macroscale (Diez et al, 2014;Holnicki and Nahorski, 2015) and at mesoscale (Saikawa et al, 2017), topography and land use data uncertainty at macroscale (Zou et al, 2016), and surface roughness uncertainty at macroscale (Barnes et al, 2014). The challenges to model inputs and processes, especially regarding the consideration of GI in air pollutant concentration simulations, primarily relate to: (i) spatio-temporal variation of GI characteristics such as shape and size, porosity, pollution tolerance and pollutant sink; (ii) pollutant transformation due to GI; and (iii) influences of meteorological and topographical data (such as temperature, humidity, terrain slope, wind speed and direction) on the deposition process.…”