Skyhook technology is widely used in vibration control. However, it only attenuates vibration near the resonant frequency. To enhance the control performance of an isolation system, a new feedforward compensation control strategy, achieved by measuring base velocity with a geophone, is proposed in this paper. Firstly, the mathematical model of single degree-of-freedom pneumatic spring is derived in detail. Secondly, the feedback controller is designed experimentally, and an anti-windup proportion-integral controller is used. Thirdly, the feedforward compensation controller is designed using a finite impulse response filter, whose coefficients are updated on-line using the filtered-x least-mean-square algorithm with improved gradient estimate. At last, a series of experiments were conducted, and the velocity attenuation rate is calculated. The results of these experiments prove that the proposed method can greatly reduce base disturbance, and keep a high vibration velocity attenuation rate at all frequency points.