Ultrafine Nanoclusters Unlocked 3d–4f Electronic Ladders for Efficient Electrocatalytic Water Oxidation
Xuemin Wang,
Na Li,
Gui-Chang Wang
et al.
Abstract:The vast extensional planes of two-dimensional (2D) nanomaterials are recognized as desirable ground for electrocatalytic reactions. However, they tend to exhibit catalytic inertia due to their surface-ordered coordination configurations. Herein, an in situ autoxidation strategy enables high-density grafting of ultrafine CeO 2 nanoclusters on 2D Co(OH) 2 . Affluent active units were activated at the inert interface of Co(OH) 2 via the formation of Co−O−Ce units. The optimized catalyst exhibits oxygen evolution… Show more
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