2022
DOI: 10.1021/acs.nanolett.2c01059
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Ultimate Limit for Optical Losses in Gold, Revealed by Quantitative Near-Field Microscopy

Abstract: We report thorough measurements of surface plasmon polaritons (SPPs) running along nearly perfect air-gold interfaces formed by atomically flat surfaces of chemically synthesized gold monocrystals. By means of amplitude-and phase-resolved near-field microscopy, we obtain their propagation length and effective mode index at visible wavelengths (532, 594, 632.8, 729, and 800 nm). The measured values are compared with the values obtained from the dielectric functions of gold that are reported in literature. Impor… Show more

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Cited by 16 publications
(15 citation statements)
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“…It should be noted that the efficiency can be further increased by using high-refractive index metasurface ridges to boost their out-of-plane scattering and high-quality monocrystalline metal films to reduce the ohmic losses [34]. Thus, simply by changing the ridge material to titanium dioxide (TiO 2 ), the external quantum efficiency is expected to exceed 80%, even without further optimization of ridge parameters as described for the bullseye pattern [23].…”
Section: Discussionmentioning
confidence: 99%
“…It should be noted that the efficiency can be further increased by using high-refractive index metasurface ridges to boost their out-of-plane scattering and high-quality monocrystalline metal films to reduce the ohmic losses [34]. Thus, simply by changing the ridge material to titanium dioxide (TiO 2 ), the external quantum efficiency is expected to exceed 80%, even without further optimization of ridge parameters as described for the bullseye pattern [23].…”
Section: Discussionmentioning
confidence: 99%
“…Highly linearity modulation response is realized by passive control of the relative phase in the nonidentical waveguides forming the interferometric arms. Optical transmission and scattering losses introduced by the isolating air gap have been characterized and can potentially be further reduced by using a high-quality (monocrystalline) Au platform for the plasmonic phase shifters 18 and by eventually interfacing the plasmonic waveguides with a low-loss photonic circuit. 24 As lithium niobate provides the critical material properties for practical deployment in electro-optic modulation applications, it remains the material-of-choice for telecommunication technology.…”
Section: ■ Discussionmentioning
confidence: 99%
“…Precise knowledge of dielectric function is crucial, e.g., for understanding the electronic structure of metals, chemical bonding, and optical properties [16][17][18][19][20][21]. The dielectric function also determines many important parameters in plasmonics [22], such as surface plasmon propagation length, plasmon radiation rate, and nonradiative losses [23][24][25].…”
Section: Introductionmentioning
confidence: 99%