A measurement procedure for the rapid acquisition of U-Pb dates for detrital zircons by quadrupole LA-ICP-MS was developed. The procedure achieves a threefold increase in measurement efficiency compared with the most commonly used methods. Utilising reduced background counting times and a shortened ablation period, a throughput of 130 measurements/h can be achieved. The measurement procedure was characterised and validated using data from thirty-nine sessions acquired over a twelve-month period. Systematic measurement error in 206 Pb/ 238 U dates for reference materials used for quality control with ages between 28.2 and 2672 Ma was < 1.5%. Average measurement uncertainty, including both random and systematic components, was 1-4% (2s). Interrogation of time-resolved calculated dates and signal intensities for each measurement allows for the detection and elimination of portions of measurements exhibiting age heterogeneities, zoning, lead loss and contamination by common lead. The measurement procedure diminishes the need to acquire cathodoluminescence imagery for routine detrital zircon applications further increasing throughput and reducing cost. The utility of the measurement procedure is demonstrated by the measurement of samples previously characterised by LA-MC-ICP-MS.Keywords: LA-ICP-MS, U-Pb geochronology, detrital zircon, data reduction.
Received 10 Feb 16 -Accepted 25 Aug 16Detrital zircon geochronology is a powerful tool for the recognition and mapping of ancient sediment dispersal systems (e.g., Rainbird et al. 1992, Gehrels and Dickinson 1995, Leier and Gehrels 2011, the characterisation of sediment source terranes (e.g., Lewis et al. 2010, Afinson et al. 2012, identifying displaced crustal fragments (e.g., Housen and Beck 1999, Garver andDavidson 2015) and for constraining the maximum depositional ages of sedimentary units (Dickinson and Gehrels 2009). Early detrital zircon U-Pb studies utilised isotope dilution-thermal ionisation mass spectrometry (ID-TIMS) of individual and multigrain zircon fractions (e.g., Girty and Wardlaw 1985, Gehrels andRoss 1998). The relatively high cost of timeintensive ID-TIMS measurements limited the number of dates incorporated in these studies. The small n (where n refers to the number of dates obtained from a single sample) of these early studies limited their statistical robustness and allowed only basic conclusions to be drawn about the sample's provenance. The advent of SIMS and LA-ICP-MS revolutionised detrital zircon geochronology by facilitating the efficient acquisition of a much larger number of measurements. In the last decade, LA-ICP-MS has become the method of choice for detrital zircon studies due to its high throughput and good spatial resolution and uncertainty (Schaltegger et al. 2015).Until recently, the majority of detrital zircon studies conducted by LA-ICP-MS reported dates for~100 individual zircons from each sample; a compromise between acquiring sufficient dates to adequately characterise a rock's provenance and the associated analytical costs...