2021
DOI: 10.1021/acs.jpclett.1c02290
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Two-Dimensional Hybrid Perovskite-Based van der Waals Heterostructures

Abstract: Figure 2. Construction routes of 2D perovskite heterostructures. (a) Schematic illustration of dry transfer method to build heterostructures.

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Cited by 21 publications
(22 citation statements)
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“…Similar to the case of perovskite solar cells, [84] the development of optoelectronic devices based on 2DP/TMD stacks significantly outpaced the understanding of their fundamental properties. Despite successful demonstrations of photodetectors or photovoltaic devises based on van der Waals heterostructures composed of 2DPs and TMDs or other layered materials, [23,24,27,[85][86][87][88][89] still very little is know about the fundamental mechanisms standing behind their operation. Most published work focuses on the device performance and only a few publications attempt to provide a more detailed understanding of the photophysics, excitation transfer mechanism and mutual impact of the layers.…”
Section: Photophysics Of 2dp/tmds Stacksmentioning
confidence: 99%
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“…Similar to the case of perovskite solar cells, [84] the development of optoelectronic devices based on 2DP/TMD stacks significantly outpaced the understanding of their fundamental properties. Despite successful demonstrations of photodetectors or photovoltaic devises based on van der Waals heterostructures composed of 2DPs and TMDs or other layered materials, [23,24,27,[85][86][87][88][89] still very little is know about the fundamental mechanisms standing behind their operation. Most published work focuses on the device performance and only a few publications attempt to provide a more detailed understanding of the photophysics, excitation transfer mechanism and mutual impact of the layers.…”
Section: Photophysics Of 2dp/tmds Stacksmentioning
confidence: 99%
“…In the next part, we summarize the current understanding of basic properties of TMD/2DP heterostructures. Works reviewing the progress in the device fabrication and performance based on such stack have recently appeared [27,28] . In this review, we focus our attention on the fundamental photophysics aspects of TMD/2DP structures.…”
Section: Introductionmentioning
confidence: 99%
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“…Singlelayer WS 2 is a direct semiconductor, which explains the PL enhancement 93 . Besides the free charge transfer, ex-citonic energy transfer from the exciton state of (C 6 H 5 C 2 H 4 NH 3 )PbI 4 to an upper-lying exciton state of WS 2 is also possible 95,155 . Interestingly, even the deeper perovskite layers contribute to the energy transfer, leading to a large enhancement of PL from WS 2 95 .…”
Section: Perovskite/tmd Heterostructuresmentioning
confidence: 99%
“…Recently, the integration of perovskite and TMDs has stimulated interest in multidisciplinary areas and holds great promise for many optoelectronic applications 89−94 . Particularly, combining the two materials together may improve the optical response of the sensitizing optical devices 93,95 .…”
Section: Introductionmentioning
confidence: 99%