Abstract:Two-dimensional electronic spectroscopy (2DES) is a powerful method to probe the coherent electron dynamics in complicated systems. Stabilizing the phase difference of the incident ultrashort pulses is the most challenging part for experimental demonstration of 2DES. Here, we present a tutorial review on the 2DES protocols based on active phase managements which are originally developed for quantum optics experiments. We introduce the 2DES techniques in box and pump-probe geometries with phase stabilization re… Show more
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