Abstract:We present Floquet calculations of the total rate for multiphoton ionization of atomic hydrogen by a coherent superposition of the second and third harmonics of a Nd:YLF (neodymium-doped yttrium-lithium-fluoride) laser Beld. The total rate depends little on the relative phase of the two 6elds in the range of intensity considered.PACS number(s): 32.80.Rm
“…Further, the relative phase dependence of the total rates is more pronounced for the frequency ratio 1:3 than for 1:2 [4] and 2:3 [5] since all the pathways leading to a continuum states with the same energy interfere in the 1:3 case whereas a considerable pattern of uninterfering pathways exists for the other cases due to parity or energy restrictions [5]. The oscillatory ionization probability dependence on the relative phase with the maximum at 5 =0 and minimum at 5 = m was also reported by Pont, Proulx, and Shakeshaft [6] [7 -9], doubly excited states far above the ionization threshold can be safely ignored for moderately strong laser fields.…”
We present a general nonperturbative formalism and an eScient and accurate numerical technique for the study of the angular distributions and partial widths for multiphoton above-threshold detachment in two-color fields. The procedure is based on an extension of our recent paper [D. A. Telnov and S.-I Chu, Phys. Rev. A 50, 4099 (1994)
“…Further, the relative phase dependence of the total rates is more pronounced for the frequency ratio 1:3 than for 1:2 [4] and 2:3 [5] since all the pathways leading to a continuum states with the same energy interfere in the 1:3 case whereas a considerable pattern of uninterfering pathways exists for the other cases due to parity or energy restrictions [5]. The oscillatory ionization probability dependence on the relative phase with the maximum at 5 =0 and minimum at 5 = m was also reported by Pont, Proulx, and Shakeshaft [6] [7 -9], doubly excited states far above the ionization threshold can be safely ignored for moderately strong laser fields.…”
We present a general nonperturbative formalism and an eScient and accurate numerical technique for the study of the angular distributions and partial widths for multiphoton above-threshold detachment in two-color fields. The procedure is based on an extension of our recent paper [D. A. Telnov and S.-I Chu, Phys. Rev. A 50, 4099 (1994)
“…Theoretical studies of the discussed phenomenon for a number of atomic systems have been carried out both within the framework of a perturbation treatment of the electromagnetic interaction of the considered atomic system with a relatively weak bichromatic laser field 20–22 and within the framework of the so‐called Keldysh–Faisal–Reiss approach 23 and its various modifications 24 when the field of one or both is strong enough so that the interaction of a detached electron being in continuous spectrum states with its parent residual atomic core may be neglected. The case of a strong bichromatic field has been studied using various completely quantum mechanical numerical simulations of the photodetachment process for various schemes of transitions in atomic systems 25, 26. For a multi‐interacting particle system, it is a rather involved problem.…”
The two parameters V 0 and are fixed by requiring V(x) to reproduce the experimentally observed ground-state ionization energy of the halide ions concerned. The potentials so generated are shown to support only one bound state in each case. The time-dependent Fourier grid Hamiltonian method is used to follow the detachment dynamics with fairly high intensities of light. The environmental effects on the dynamics are sought to be modeled by allowing the well depth (V 0 ) to fluctuate randomly (V 0 (t) ϭ V 0 [1 ϩ ⌬VR(t)]; R(t) randomly fluctuates between ϩ1 and Ϫ1 with time, when ⌬V is fixed). The average detachment rate constants k av are seen to increase with increase in the intensities of used bichromatic field. An alternative model potential, V(x) ϭ ϪV 0 e Ϫx , is also shown to yield similar results.
“…Afterwards, a broad variety of perturbative [22,23,24,25] as well as non-perturbative results [26,27,28,29,30,31,32] has been obtained. In addition, extensive numerical investigations have also been performed [33,34,35,36,37,38,39,40].…”
We analyze atomic photoelectron momentum distributions induced by bichromatic and monochromatic laser fields within the strong field approximation (SFA), separable Coulomb-Volkov approximation (SCVA), and ab initio treatment. We focus on the high frequency regime -the smallest frequency used is larger than the ionization potential of the atom. We observe a remarkable agreement between the ab initio and velocity gauge SFA results while the velocity gauge SCVA fails to agree. Reasons of such a failure are discussed.
scite is a Brooklyn-based organization that helps researchers better discover and understand research articles through Smart Citations–citations that display the context of the citation and describe whether the article provides supporting or contrasting evidence. scite is used by students and researchers from around the world and is funded in part by the National Science Foundation and the National Institute on Drug Abuse of the National Institutes of Health.