We report on ordered nanoporous films exhibiting a unique magneto-plasmon based response, fabricated by nanosphere-assisted physical deposition. This work focuses on multi-layer Ag/CoFeB/Ag films as examples of such structures. Their microstructure dependent magnetic properties, localized surface plasmon resonance (LSPR) and magneto-optical Kerr effect were investigated. The observed effects of nanopores and Ag layers on the magnetic properties indicate the synergistic interaction between nanopores and Ag layers leading to an enhancement of the ferromagnetic character of the CoFeB film. LSPR spectra reveal that the introduction of Ag layers enhances the light transmission in the nanoporous CoFeB films (having pore sizes exceeding the wavelength of light) due to an enhanced interaction of light with surface plasmons. Periodic nanoporous Ag/CoFeB/Ag films covered by Ag capped nanospheres show a much larger extinction than uncovered nanoporous Ag/CoFeB/Ag films. The correlation between the magneto-optical Kerr effect and the nanostructures suggests a field-tunable Kerr effect owing to the magneto-electric coupling between the magnetic layer and the Ag layers, which is enhanced by the nanopores. These hybrid nanostructures are expected to offer potential applications in photovoltaic cells and for magneto-optic sensors.H ybridization of nanostructures has emerged as a new way of realizing multi-functionality and/or improved physical and chemical properties arising from the coupling of constituent materials (e.g. interfacial magneto-electric coupling or IFMEC) [1][2][3][4][5][6][7][8][9][10][11][12][13] . This innovative approach also offers a route for overcoming undesirable compromises between material properties and performance that accompany size reduction in nanotechnology. Examples include increased activity but reduced stability [5][6][7][14][15][16][17][18] , superparamagnetism versus ferromagnetism 3,19 , increased sensitivity but reduced intensity 11,[20][21][22] , and enhanced magneto-optical effect but increased energy loss 23,24 . Applications of new types of multi-functional nanoparticles (NPs) based on hybridization require control over the mismatch among different components and a good understanding of the interface-coupling and proximity effects in the constituent parts 3,5,7,8,25 . It is also essential to develop controlled processes for large scale fabrication of well-defined nanoentities with long-term stability in desired media 10,[26][27][28][29][30][31][32][33][34][35] .For hybrid nanomaterials with magnetic components, both the magnetic properties and dielectric constants can be tuned by IFMEC effects, leading to enhanced magnetic, electronic, optical and acoustic properties 1,5,23,24 . Recent investigations indicate that active magneto-plasmonic nanomaterials formed by noble metals and magnetic metals can improve the interaction between magnetic field, electric field, electromagnetic waves and the localized surface plasmon resonance (LSPR), leading to applications for efficient switching and t...