Trivalent Cation Defect Optimization Spin State of Nickel(II) in NiFe-Layered Double Hydroxide Nanosheets for Oxygen Evolution
Xiaobao Zhang,
Haohai Dong,
Haomin Jiang
et al.
Abstract:The defects have been confirmed to activate catalytic sites and significantly enhance electrocatalytic activity. However, the influence of defects on the electronic spin state of catalytic active sites and their impact on catalytic behavior are still in the early stages of research. Spin behavior is a fundamental property of the electrons. Herein, using NiFe-LDH nanosheets as the model structure, we constructed trivalent cation vacancy models to gain a deeper understanding of the intrinsic relationship among d… Show more
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