Abstract:[1] The six longest records of stratospheric aerosol (in situ measurements at Laramie, Wyoming, lidar records at: Garmisch-Partenkirchen, Germany; Hampton, Virginia; Mauna Loa, Hawaii; São José dos Campos, Brazil, and SAGE II measurements) were investigated for trend by (1) comparing measurements in the 3 volcanically quiescent periods since 1970 using standard analysis of variance techniques, and (2) analyzing residuals from a time/volcano dependent empirical model applied to entire data sets. A standard squa… Show more
“…Since 1972, time series have been obtainable from lidar measurements, balloon ascents (Hofmann et al, 1975), and also satellite observations (McCormick et al, 1981;Thomason et al, 1987). For recent reviews see Deshler et al (2006) and Deshler (2008). These observations, covering a number of important eruptions, have led to clear evidence of the mainly volcanic nature of the stratospheric aerosol.…”
Section: T Trickl Et Al: Stratospheric Aerosol: From Fuego To Eyjafmentioning
confidence: 99%
“…A scientific summary for the period 1976-1999 was given by Jäger (2005). Deshler et al (2006) and Deshler (2008) compared the results with those from the most important stations performing stratospheric aerosol sounding.…”
Section: T Trickl Et Al: Stratospheric Aerosol: From Fuego To Eyjafmentioning
confidence: 99%
“…The lidar system at IMK-IFU is an instrument of both NDACC and EARLINET. This system was originally built in 1973 (Impulsphysik GmbH), based on a ruby laser, and, in addition to a large number of routine and campaign-type tropospheric measurements (e.g., Reiter and Carnuth, 1975 Jäger et al, 1988Jäger et al, , 2006Forster et al, 2001;Trickl et al, 2003Trickl et al, , 2011, has been almost continually used for measurements of stratospheric aerosol since autumn 1976 (e.g., Jäger, 2005;Deshler et al, 2006;Fromm et al, 2008bFromm et al, , 2010. The lidar was converted to a spatially scanning system with a Nd:YAG laser (Quanta Ray, GCR 4, 10 Hz repetition rate, about 700 mJ per pulse at 532 nm) in the early 1990s for additional investigation of contrails (Freudenthaler, 2000;Freudenthaler et al, 1994Freudenthaler et al, , 1995.…”
Lidar measurements at Garmisch-Partenkirchen (Germany) have almost continually delivered backscatter coefficients of stratospheric aerosol since 1976. The time series is dominated by signals from the particles injected into or formed in the stratosphere due to major volcanic eruptions, in particular those of El Chichon (Mexico, 1982) and Mt Pinatubo (Philippines, 1991). Here, we focus more on the long-lasting background period since the late 1990s and 2006, in view of processes maintaining a residual lower-stratospheric aerosol layer in absence of major eruptions, as well as the period of moderate volcanic impact afterwards. During the long background period the stratospheric backscatter coefficients reached a level even below that observed in the late 1970s. This suggests that the predicted potential influence of the strongly growing air traffic on the stratospheric aerosol loading is very low. Some correlation may be found with single strong forest-fire events, but the average influence of biomass burning seems to be quite limited. No positive trend in background aerosol can be resolved over a period as long as that observed by lidar at Mauna Loa. We conclude that the increase of our integrated backscatter coefficients starting in 2008 is mostly due to volcanic eruptions with explosivity index 4, penetrating strongly into the stratosphere. Most of them occurred in the mid-latitudes. A key observation for judging the role of eruptions just reaching the tropopause region was that of the plume from the Icelandic volcano Eyjafjallajökull above Garmisch-Partenkirchen (April 2010) due to the proximity of that source. The top altitude of the ash above the volcano was reported just as 9.3 km, but the lidar measurements revealed enhanced stratospheric aerosol up to 14.3 km. Our analysis suggests for two or three of the four measurement days the presence of a stratospheric contribution from Iceland related to quasi-horizontal transport, differing from the strong descent of the layers entering Central Europe at low altitudes. The backscatter coefficients within the first 2 km above the tropopause exceed the stratospheric background by a factor of four to five. In addition, Asian and Saharan dust layers were identified in the free troposphere, Asian dust most likely even in the stratosphere
“…Since 1972, time series have been obtainable from lidar measurements, balloon ascents (Hofmann et al, 1975), and also satellite observations (McCormick et al, 1981;Thomason et al, 1987). For recent reviews see Deshler et al (2006) and Deshler (2008). These observations, covering a number of important eruptions, have led to clear evidence of the mainly volcanic nature of the stratospheric aerosol.…”
Section: T Trickl Et Al: Stratospheric Aerosol: From Fuego To Eyjafmentioning
confidence: 99%
“…A scientific summary for the period 1976-1999 was given by Jäger (2005). Deshler et al (2006) and Deshler (2008) compared the results with those from the most important stations performing stratospheric aerosol sounding.…”
Section: T Trickl Et Al: Stratospheric Aerosol: From Fuego To Eyjafmentioning
confidence: 99%
“…The lidar system at IMK-IFU is an instrument of both NDACC and EARLINET. This system was originally built in 1973 (Impulsphysik GmbH), based on a ruby laser, and, in addition to a large number of routine and campaign-type tropospheric measurements (e.g., Reiter and Carnuth, 1975 Jäger et al, 1988Jäger et al, , 2006Forster et al, 2001;Trickl et al, 2003Trickl et al, , 2011, has been almost continually used for measurements of stratospheric aerosol since autumn 1976 (e.g., Jäger, 2005;Deshler et al, 2006;Fromm et al, 2008bFromm et al, , 2010. The lidar was converted to a spatially scanning system with a Nd:YAG laser (Quanta Ray, GCR 4, 10 Hz repetition rate, about 700 mJ per pulse at 532 nm) in the early 1990s for additional investigation of contrails (Freudenthaler, 2000;Freudenthaler et al, 1994Freudenthaler et al, , 1995.…”
Lidar measurements at Garmisch-Partenkirchen (Germany) have almost continually delivered backscatter coefficients of stratospheric aerosol since 1976. The time series is dominated by signals from the particles injected into or formed in the stratosphere due to major volcanic eruptions, in particular those of El Chichon (Mexico, 1982) and Mt Pinatubo (Philippines, 1991). Here, we focus more on the long-lasting background period since the late 1990s and 2006, in view of processes maintaining a residual lower-stratospheric aerosol layer in absence of major eruptions, as well as the period of moderate volcanic impact afterwards. During the long background period the stratospheric backscatter coefficients reached a level even below that observed in the late 1970s. This suggests that the predicted potential influence of the strongly growing air traffic on the stratospheric aerosol loading is very low. Some correlation may be found with single strong forest-fire events, but the average influence of biomass burning seems to be quite limited. No positive trend in background aerosol can be resolved over a period as long as that observed by lidar at Mauna Loa. We conclude that the increase of our integrated backscatter coefficients starting in 2008 is mostly due to volcanic eruptions with explosivity index 4, penetrating strongly into the stratosphere. Most of them occurred in the mid-latitudes. A key observation for judging the role of eruptions just reaching the tropopause region was that of the plume from the Icelandic volcano Eyjafjallajökull above Garmisch-Partenkirchen (April 2010) due to the proximity of that source. The top altitude of the ash above the volcano was reported just as 9.3 km, but the lidar measurements revealed enhanced stratospheric aerosol up to 14.3 km. Our analysis suggests for two or three of the four measurement days the presence of a stratospheric contribution from Iceland related to quasi-horizontal transport, differing from the strong descent of the layers entering Central Europe at low altitudes. The backscatter coefficients within the first 2 km above the tropopause exceed the stratospheric background by a factor of four to five. In addition, Asian and Saharan dust layers were identified in the free troposphere, Asian dust most likely even in the stratosphere
“…These measurements will be used (in this study) as prior knowledge, with the help of which SAGE II spectral extinction measurements will be evaluated to obtain new estimates of aerosol properties under non-volcanic conditions. The balloone-borne measurements from Laramie along with ground based lidar measurements at two mid-latitude sites (Osborn et al, 1995;Jäger, 2005) and two tropical sites (Barnes and Hofmann, 1997;Simonich and Clemesha, 1997) provide the longest stratospheric aerosol records available (Deshler et al, 2006). They are particularly valuable, for instance, for having captured the complete cycle of three major volcanic eruptions (Fuego, 1974, 14 • N;El Chichón, 1982, 17 • N;Pinatubo, 1991, 15 • N) which have not been measured in as much detail or even not at all by satellite instruments.…”
Abstract. Stratospheric aerosol particles under non-volcanic conditions are typically smaller than 0.1 µm. Due to fundamental limitations of the scattering theory in the Rayleigh limit, these tiny particles are hard to measure by satellite instruments. As a consequence, current estimates of global aerosol properties retrieved from spectral aerosol extinction measurements tend to be strongly biased. Aerosol surface area densities, for instance, are observed to be about 40% smaller than those derived from correlative in situ measurements . An accurate knowledge of the global distribution of aerosol properties is, however, essential to better understand and quantify the role they play in atmospheric chemistry, dynamics, radiation and climate.To address this need a new retrieval algorithm was developed, which employs a nonlinear Optimal Estimation (OE) method to iteratively solve for the monomodal size distribution parameters which are statistically most consistent with both the satellite-measured multi-wavelength aerosol extinction data and a priori information. By thus combining spectral extinction measurements (at visible to near infrared wavelengths) with prior knowledge of aerosol properties at background level, even the smallest particles are taken into account which are practically invisible to optical remote sensing instruments.The performance of the OE retrieval algorithm was assessed based on synthetic spectral extinction data generated from both monomodal and small-mode-dominant bimodal sulphuric acid aerosol size distributions. For monomodal background aerosol, the new algorithm was shown to fairly Correspondence to: D. Wurl (daniela wurl@yahoo.de) accurately retrieve the particle sizes and associated integrated properties (surface area and volume densities), even in the presence of large extinction uncertainty. The associated retrieved uncertainties are a good estimate of the true errors. In the case of bimodal background aerosol, where the retrieved (monomodal) size distributions naturally differ from the correct bimodal values, the associated surface area (A) and volume densities (V ) are, nevertheless, fairly accurately retrieved, except at values larger than 1.0 µm 2 cm −3 (A) and 0.05 µm 3 cm −3 (V ), where they tend to underestimate the true bimodal values. Due to the limited information content in the SAGE II spectral extinction measurements this kind of forward model error cannot be avoided here. Nevertheless, the retrieved uncertainties are a good estimate of the true errors in the retrieved integrated properties, except where the surface area density exceeds the 1.0 µm 2 cm −3 threshold.When applied to near-global SAGE II satellite extinction measured in 1999 the retrieved OE surface area and volume densities are observed to be larger by, respectively, 20-50% and 10-40% compared to those estimates obtained by the SAGE II operational retrieval algorithm. An examination of the OE algorithm biases with in situ data indicates that the new OE aerosol property estimates tend to be more realistic tha...
“…In situ balloon observations continue to be used and have provided highly valuable data sets, including most notably the long time series of optical particle counter measurements from Laramie, WY (Deshler et al, 2003(Deshler et al, , 2006Kovilakam and Deshler, 2015). Aircraft-borne nephelometers (Beuttell and Brewer, 1949;Charlson et al, 1969) acquire detailed in situ measurements, providing, for example, plume composition (Murphy et al, 2014), but are spatially limited to the aircraft track.…”
Abstract. The Aerosol Limb Imager (ALI) is an optical remote sensing instrument designed to image scattered sunlight from the atmospheric limb. These measurements are used to retrieve spatially resolved information of the stratospheric aerosol distribution, including spectral extinction coefficient and particle size. Here we present the design, development and test results of an ALI prototype instrument. The longterm goal of this work is the eventual realization of ALI on a satellite platform in low earth orbit, where it can provide high spatial resolution observations, both in the vertical and cross-track. The instrument design uses a large-aperture acousto-optic tunable filter (AOTF) to image the sunlit stratospheric limb in a selectable narrow wavelength band ranging from the visible to the near infrared. The ALI prototype was tested on a stratospheric balloon flight from the Canadian Space Agency (CSA) launch facility in Timmins, Canada, in September 2014. Preliminary analysis of the hyperspectral images indicates that the radiance measurements are of high quality, and we have used these to retrieve vertical profiles of stratospheric aerosol extinction coefficient from 650 to 1000 nm, along with one moment of the particle size distribution. Those preliminary results are promising and development of a satellite prototype of ALI within the Canadian Space Agency is ongoing.
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