The 22nd International Conference on Ultrafast Phenomena 2020 2020
DOI: 10.1364/up.2020.m4b.10
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Tracking Ultrafast Charge Separation in a PBI-based Biomimetic Complex for Oxygen Evolution

Abstract: Multidimensional spectroscopies reveal a two-step process in a biomimetic supracomplex for oxygen evolution. A sub-ps charge-separation within the light-sensitizer moiety is followed by hole transfer from the catalyst counterpart, forming productive charges.

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