Abstract:Timeresolved infrared diode laser spectroscopy of the ν5 band of the cyanomethyl radical (H2CCN)The time-resolved spectral output of a pulsed H2"Fz laser has been investigated as a function of initiating atomic fluorine concentration. Fast initiation, as well as variation of initial F-atom concentration. was accomplished by photodissociation of F z in a flowing Hz-Fz-N z mixture utilizing a variable-amplitude 30-nsee second harmonic pulse from a Q -switched ruby laser. Initial HF concentration due to prereacti… Show more
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