Fluidized bed membrane reactors have been introduced
in catalytic
reforming hydrogen production recently. The arrangement of membrane
tubes is the key factor in the gas–solid distribution in reactors,
which decides the production efficiency and wearing characteristics
of membrane tubes. Nevertheless, research on optimization of the arrangement
of membrane tubes is still inadequate due to a lack of measuring methods
which can penetrate solid particles and internal components. In this
study, the time-averaged void fraction distributions inside fluidized
bed membrane reactors with different fluidization velocities and tube
layouts are investigated using X-ray computed tomography. The effects
of spacers on the internal gas–solid flow characteristics are
studied as well. The results indicate that bubbles first gather toward
the bed center axis during rising, then cut by the tube bundle, causing
bubbles to split and then aggregate. Increasing the number of bundles
makes the distribution of bubbles more uniform. The spacer allows
more bubbles to move along the wall, and these bubbles tend to return
to the middle of the fluidized bed after passing through the spacer,
leading to more particle aggregation around the spacer. Using a multibundle
spacer can reduce aggregation. As the bed height increases, the void
fraction at the wall of the fluidized bed is less affected by the
number of tube bundles, and the use of spacers strengthens the positive
impact of the number of tube bundles. As the fluidization velocity
increases, bubbles gather toward the bed center. The presence of tube
bundles will cause the accumulation of bubbles to be more rapid.