Three-Dimensional Dual-Site Catalysts for Industrial Ammonia Synthesis at Dramatically Decreased Temperatures and Pressures
Xingshuai Lv,
Junxian Liu,
Liangzhi Kou
et al.
Abstract:Industrial ammonia (NH 3 ) production via the Haber−Bosch (H−B) process is a great achievement of the 20th century, but its energy-intensive character renders NH 3 production costly. Despite considerable efforts, progress in developing an efficient H−B catalyst that operates under near-ambient conditions has been slow. In this study, we leverage the confinement concept to facilitate low-temperature and low-pressure NH 3 synthesis by constructing three-dimensional (3D) dual-site environments. Through first-prin… Show more
“…These findings further support the high experimental feasibility of these complexes. 73 Moreover, electrical conductivity analysis is needed to investigate their electrocatalysis potential. As shown in Fig.…”
A systematic investigation using first principles calculations has explored the electrocatalytic potential of eleven main-group metal-doped blue phosphorene (M-BPs) for the oxygen evolution reaction (OER) and hydrogen evolution reaction (HER)....
“…These findings further support the high experimental feasibility of these complexes. 73 Moreover, electrical conductivity analysis is needed to investigate their electrocatalysis potential. As shown in Fig.…”
A systematic investigation using first principles calculations has explored the electrocatalytic potential of eleven main-group metal-doped blue phosphorene (M-BPs) for the oxygen evolution reaction (OER) and hydrogen evolution reaction (HER)....
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