“…Here we explore up-conversion processes in a crystal with isotopically purified 170 Er dopants at low temperatures (<1 K) using a single optical pass through the sample. Models suggest that with an optical resonator it is ultimately possible to achieve efficiencies of around 80% in this regime [36]. Our measurements are qualitatively compared with the predictions of these models, using Raman heterodyne spectroscopy with the spins being probed strongly coupled to a microwave resonator.…”
Section: Introductionmentioning
confidence: 90%
“…The individual ions are modeled using methods described in Refs. [30,36]. Because there is no cavity enhancement of the optical output field, this field will have a very small amplitude and we assume that this field does not drive the ions.…”
Raman heterodyne spectroscopy is a powerful tool for characterizing the energy and dynamics of spins. The technique uses an optical pump to transfer coherence from a spin transition to an optical transition where the coherent emission is more easily detected. Here Raman heterodyne spectroscopy is used to probe an isotopically purified ensemble of erbium dopants in a yttrium orthosilicate (Y 2 SiO 5 ) crystal coupled to a microwave cavity. Because the erbium electron spin transition is strongly coupled to the microwave cavity, we observed Raman heterodyne signals at the resonant frequencies of the hybrid spin-cavity modes (polaritons) rather than the bare erbium spin-transition frequency. Using the coupled system, we made saturation recovery measurements of the ground-state spin relaxation time T 1 = 10 ± 3 s and also observed Raman heterodyne signals using an excited state spin transition. We discuss the implications of these results for efforts toward converting microwave quantum states to optical quantum states.
“…Here we explore up-conversion processes in a crystal with isotopically purified 170 Er dopants at low temperatures (<1 K) using a single optical pass through the sample. Models suggest that with an optical resonator it is ultimately possible to achieve efficiencies of around 80% in this regime [36]. Our measurements are qualitatively compared with the predictions of these models, using Raman heterodyne spectroscopy with the spins being probed strongly coupled to a microwave resonator.…”
Section: Introductionmentioning
confidence: 90%
“…The individual ions are modeled using methods described in Refs. [30,36]. Because there is no cavity enhancement of the optical output field, this field will have a very small amplitude and we assume that this field does not drive the ions.…”
Raman heterodyne spectroscopy is a powerful tool for characterizing the energy and dynamics of spins. The technique uses an optical pump to transfer coherence from a spin transition to an optical transition where the coherent emission is more easily detected. Here Raman heterodyne spectroscopy is used to probe an isotopically purified ensemble of erbium dopants in a yttrium orthosilicate (Y 2 SiO 5 ) crystal coupled to a microwave cavity. Because the erbium electron spin transition is strongly coupled to the microwave cavity, we observed Raman heterodyne signals at the resonant frequencies of the hybrid spin-cavity modes (polaritons) rather than the bare erbium spin-transition frequency. Using the coupled system, we made saturation recovery measurements of the ground-state spin relaxation time T 1 = 10 ± 3 s and also observed Raman heterodyne signals using an excited state spin transition. We discuss the implications of these results for efforts toward converting microwave quantum states to optical quantum states.
“…Future quantum networks may bring tremendous improvement to realms of secure communication, distributed quantum computing, and remote quantum sensing . In order for quantum networks to achieve reliable information transfer over long distances with suitable bandwidth, the network nodes must eventually employ quantum repeaters to overcome lossy single photon channels. − Trivalent erbium (Er 3+ or Er for brevity) is a workhorse emitter used in traditional telecommunications technology, and Er ions have recently emerged as promising communication qubits due to their narrow telecom C-band optical transition , and long electron spin coherence times. − Individual Er ions have already shown promise as a quantum memory element in repeaters, demonstrating storage via the spin state for use in future entanglement swapping protocols. − In addition, photonics-integrated ensembles of Er ions have also been applied in microwave-to-optical quantum state transduction, − to address the challenge of interfacing the optical photons used in quantum networks (∼195 THz) with processing nodes operating at microwave frequencies (∼10 GHz). However, despite these benefits, the long-lived optical lifetime of the telecom C-band transition has limited its development as nanophotonic cavities are necessary to enhance light–matter interactions and greatly decrease the photon excited state lifetime via Purcell enhancement.…”
mentioning
confidence: 99%
“… 8 − 10 Individual Er ions have already shown promise as a quantum memory element in repeaters, demonstrating storage via the spin state for use in future entanglement swapping protocols. 11 − 13 In addition, photonics-integrated ensembles of Er ions have also been applied in microwave-to-optical quantum state transduction, 14 − 16 to address the challenge of interfacing the optical photons used in quantum networks (∼195 THz) with processing nodes operating at microwave frequencies (∼10 GHz). However, despite these benefits, the long-lived optical lifetime of the telecom C-band transition has limited its development as nanophotonic cavities are necessary to enhance light–matter interactions and greatly decrease the photon excited state lifetime via Purcell enhancement.…”
The use of trivalent erbium (Er3+), typically
embedded
as an atomic defect in the solid-state, has widespread adoption as
a dopant in telecommunication devices and shows promise as a spin-based
quantum memory for quantum communication. In particular, its natural
telecom C-band optical transition and spin-photon interface make it
an ideal candidate for integration into existing optical fiber networks
without the need for quantum frequency conversion. However, successful
scaling requires a host material with few intrinsic nuclear spins,
compatibility with semiconductor foundry processes, and straightforward
integration with silicon photonics. Here, we present Er-doped titanium
dioxide (TiO2) thin film growth on silicon substrates using
a foundry-scalable atomic layer deposition process with a wide range
of doping controls over the Er concentration. Even though the as-grown
films are amorphous after oxygen annealing, they exhibit relatively
large crystalline grains, and the embedded Er ions exhibit the characteristic
optical emission spectrum from anatase TiO2. Critically,
this growth and annealing process maintains the low surface roughness
required for nanophotonic integration. Finally, we interface Er ensembles
with high quality factor Si nanophotonic cavities via evanescent coupling
and demonstrate a large Purcell enhancement (≈300) of their
optical lifetime. Our findings demonstrate a low-temperature, nondestructive,
and substrate-independent process for integrating Er-doped materials
with silicon photonics. At high doping densities this platform can
enable integrated photonic components such as on-chip amplifiers and
lasers, while dilute concentrations can realize single ion quantum
memories.
scite is a Brooklyn-based organization that helps researchers better discover and understand research articles through Smart Citations–citations that display the context of the citation and describe whether the article provides supporting or contrasting evidence. scite is used by students and researchers from around the world and is funded in part by the National Science Foundation and the National Institute on Drug Abuse of the National Institutes of Health.