Giant magnetoelectric (ME) voltage and charge coefficients have been found in long-type composites of high-permeability magnetostrictive FeBSiC alloy ribbons laminated together with piezoelectric Pb(Zn1∕3,Nb2∕3)O3–7%PbTiO3 single crystal fibers. The maximum ME voltage and charge coefficients at low frequencies were 10.5V∕cmOe and 1nC∕Oe under a notably low dc magnetic bias of 2Oe; at resonance, these coefficients were dramatically increased to 400V∕cmOe and 42nC∕Oe, respectively. These values are much higher, and the required dc magnetic bias much lower, than those of previously reported Terfenol-D based ME laminates.