Theory of lasing in a two-dimensional array of plasmonic nanolasers

Abstract

A theory of lasing in a two-dimensional array of metal nanoparticles (MNPs) covered with a thin layer of fluorescent molecules is developed from first principles. The approach is based on a rigorous account of the local field in a close vicinity of a reflective surface which provides a feedback for molecular dipole oscillations. The theory predicts the lasing threshold in such an open cavity in terms of the polar angle of laser emission, MNPs shape and the molecular layer thickness. It is demonstrated that the latter parameter plays a crucial role in the lasing condition and controls a switching from conventional lasing to lasing without inversion. This research is inspired by recent experiments in this field [N. Toropov et al, Adv. Photonics Res. 2, 2000083 (2021)] and provides the numerical calculations carried out for the experimental conditions.