Abstract. Numerous studies have reported that ambient air pollution, which has both
local and long-range sources, causes adverse impacts on the environment and
human health. Previous studies have investigated the impacts of
transboundary air pollution (TAP) in East Asia, albeit primarily through
analyses of episodic events. In addition, it is useful to better understand
the spatiotemporal variations in TAP and the resultant impact on the
environment and human health. This study aimed at assessing and
quantifying the air quality impacts in Japan and South Korea due to local emissions and TAP from sources in East Asia - one of the most polluted
regions in the world. We applied state-of-the-science atmospheric
models to simulate air quality in East Asia and then analyzed the air
quality and acid deposition impacts of both local emissions and TAP sources
in Japan and South Korea. Our results show that ∼ 30 % of
the annual average ambient PM2.5 concentrations in Japan and South
Korea in 2010 were contributed to by local emissions within each country, while
the remaining ∼ 70 % were contributed to by TAP from other
countries in the region. More detailed analyses also revealed that the local
contribution was higher in the metropolises of Japan (∼ 40 %–79 %) and South Korea (∼ 31 %–55 %) and that minimal
seasonal variations in surface PM2.5 occurred in Japan, whereas there was a
relatively large variation in South Korea in the winter. Further, among all
five studied anthropogenic emission sectors of China, the industrial sector
represented the greatest contributor to annual surface PM2.5
concentrations in Japan and South Korea, followed by the residential and
power generation sectors. Results also show that TAP's impact on acid
deposition (SO42- and NO3-) was larger than TAP's impact
on PM2.5 concentrations (accounting for over 80 % of the total
deposition), and that seasonal variations in acid deposition were similar
for both Japan and South Korea (i.e., higher in both the winter and summer).
Finally, wet deposition had a greater impact on mixed forests in Japan and
savannas in South Korea. Given these significant impacts of TAP in the
region, it is paramount that cross-national efforts should be taken to mitigate air
pollution problems across East Asia.