“…Recent developments in nanotechnology have demonstrated the potential of aluminum oxide or alumina (Al 2 O 3 ) for various applications due to its good chemical stability, wide band gap, and biological compatibility. − Special attention is drawn to alumina in aqueous environments, as the behavioral understanding of this solid–liquid interface is crucial for dielectric nanocomposites, water filtration, drug delivery, biosensing devices, combustion, among others. − In particular, the new developments in anodic alumina membranes, enabled by the progress in nanofabrication techniques, could be beneficial for filtration and separation of molecules, cells, or proteins, and evaporation in thermal management applications, see Figure (a). − Characterizing and tuning the inner nanopore geometry and electrostatic properties in alumina membranes facilitate molecular filtration, , while the interplay between the nanopore surface and the absorbed liquid thin film is critical for the evaporation performance . It has been suggested that most of the interfacial transport (specifically momentum and thermal) is strongly influenced by a thin layer, which usually encompasses no more than a few nanometers from the interfacial region. , Due to the reduced scale, the thickness of this region hinders accurate probing using the current experimental capabilities; therefore, atomistic-level simulations can provide useful insight into the interface and transport properties.…”