The Role of the Molecular Encapsulation Effect in Stabilizing Hydrogen‐Bond‐Rich Gel‐State Lithium Metal Batteries
Hantao Xu,
Wei Deng,
Lei Shi
et al.
Abstract:Gel‐state polymer electrolytes with superior mechanical properties, self‐healing abilities and high Li+ transference numbers can be obtained by in situ polymerization of monomers with hydrogen‐bonding moieties. However, it is overlooked that the active hydrogen atoms in hydrogen‐bond donors experience displacement reactions with lithium metal in lithium metal batteries (LMBs), leading to corrosion of the lithium metal. Herein, it is discovered that the addition of hydrogen‐bond acceptors to hydrogen‐bond‐rich … Show more
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