The relevance of structural variability in the time-domain for computational reflection anisotropy spectroscopy at solid–liquid interfaces
Justus Leist,
Jongmin Kim,
Holger Euchner
et al.
Abstract:In electrochemistry, reactions and charge-transfer are to a large extent determined by the atomistic structure of the solid-liquid interface. Yet due to the presence of the liquid electrolyte, many surface-science methods cannot be applied here. Hence, the exact microscopic structure that is present under operating conditions often remains unknown. Reflection anisotropy spectroscopy (RAS) is one of the few techniques that allow for an in operando investigation of the structure of solid-liquid interfaces. Howev… Show more
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