1957
DOI: 10.1021/ja01560a058
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The Reduction of Thioketones by a Model for a Coenzyme

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Cited by 161 publications
(46 citation statements)
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“…References to both opposing views are presented in several stimulating publications but differences in interpretation still persist [27][28][29][30][31][32][33][34][35].…”
Section: Methodsmentioning
confidence: 99%
See 1 more Smart Citation
“…References to both opposing views are presented in several stimulating publications but differences in interpretation still persist [27][28][29][30][31][32][33][34][35].…”
Section: Methodsmentioning
confidence: 99%
“…Still, we believed that evidence of semiquinone radical formation in biochemical reactions was insufficient. It seemed that the investigation of a relevant redox process such as the reaction of naturally occuring quinones with NAD(P)H models under conditions aimed to mimic those in biological systems, might be an adequate reaction although earlier examinations led to contradictiory conclusions (see above, [27][28][29][30][31][32][33][34][35]). …”
Section: Dna Damagementioning
confidence: 99%
“…The involvement of the active-site zinc ion as a Lewis acid catalyst of ternary-complex interconversion has been suggested by several authors [6,[22][23][24][25][26][27][28][29][30]. Most proposals in that direction have focused on the process of aldehyde reduction and emphasized the polarizing effect of the zinc ion on the metal-bound substrate.…”
Section: Tlzc Cntcilytic Functioti O F Thc Active-site Zinc Ionmentioning
confidence: 99%
“…from dihydronicotinamides to flavin was later formulated to involve preequilibrium complex formation along the reaction path. This was based on the lack of correlation of log(kr te) for the redox reaction with the E112 potentials for a series of flavins and the good correlation between log(krale) with log(Ke) for complex formation ofthe flavins with tryptophan (7,8 (19)(20)(21)(22)(23)(24). A multistep rather than a single-step Htransfer has been suggested in order.…”
mentioning
confidence: 99%