Abstract:. Can. J . Chem. 65, 2478Chem. 65, (1987. The microwave spectra of 79BrSCN and "B~SCN have been measured and analysed to give rotational, centrifugal distortion, and Br quadrupole coupling constants. The molecule has been shown unambiguously to be BrSCN rather than BrNCS. A harmonic force field has been determined from combined vibrational and distortion data. With structural parameters for the SCN chain transferred from S(CN)>, both effective and ground state average values for the BrS length and BrSC angle… Show more
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