Extensive carbonate crusts discovered forming on the slopes of seamounts in many parts of the world's oceans are providing extra stability to the volcanic edifices. These crusts are composed of mixtures of volcaniclastic debris and bioclastic material, in most cases cemented by calcite, in the form of isopachous coatings around grains and pore-filling spar.Such crusts, which have been collected by remotely-operated vehicle (ROV), are described here from moderate-depth to deeper-water slopes (200 -1000 m) around the volcanic island of Montserrat in the Caribbean, and from the nearby Kick'em Jenny submarine volcano off Grenada. Radiogenic 87 Sr /86 Sr isotope ratios from the carbonates give an indication of age but also demonstrate that some samples have been altered by hydrothermal-volcanic processes, as shown by ages much older than expected. Such alteration is also supported by carbon and oxygen isotope ( 13 C and 18 O) ratios, although most samples have typical marine values. In many cases 18 O is usually a little more positive than expected from modern shallow-water carbonates, likely reflecting cooler water at the depth of lithification. Just one sample, from Kick'em Jenny, has very negative 13 C (-42 ‰) indicating methanogenesis. Crusts are also reported here from the Mediterranean Sea, with an example described from Kolumbo, northeast of the Santorini volcanic complex in the Hellenic subduction zone, that are similar in many respects to those from the Caribbean. Typically, the biota of the crusts consists of calcareous red algae (commonly encrusting volcanic clasts), benthic (also encrusting) and planktic foraminifera, subordinate serpulids, bivalves, pteropods and heteropods, and rare deeper-water corals. In addition, there is evidence for the former presence of microbes from the occurrence of calcified filaments and peloids in intragranular cavities. Several generations of sponge borings are usually present as well as calcite cement. The carbonate crusts are attributed to seawater circulating within the surficial sediment, in some cases mixing with hydrothermal fluid. The significance of these crusts is in stabilising seamounts, enabling their 3 slopes to avoid frequent collapse, dissection and readjustment, but when failure does occur, larger-scale submarine landslides involving coherent slabs are more likely.