The effect of secondary capping on the control of phosphorus release from sediment by activated thin-layer capping with Al-PIA

Zhu, Bolin; Li, Shuwen; Lin, Canyang; Liu, Shupo; Li, Fēi; Zhou, Zhenming

doi:10.1007/s11356-020-11828-3

Cited by 8 publications

(1 citation statement)

References 49 publications

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“…Laboratory simulation experiments were conducted in two tanks containing mud (15 L) and water (60 L) in a 1:4 ratio, with lanthanum-modified fly ash pellets added to one tank and the other used as a blank control [55,56]. The simulated experimental setup is shown in Figure 2.…”

Section: Study Of Lanthanum Modified Fly Ash Pellets To Control Endog...mentioning

confidence: 99%

Control of Endogenous Phosphorus Release at the Sediment–Water Interface by Lanthanum-Modified Fly Ash

Pan

Liu²,

Chai

et al. 2022

Coatings

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This study optimizes the modification and granulation of fly ash to make it more stable at the sediment–water interface. Through laboratory simulations, the modified fly ash pellets were optimally granulated to cover the sediment–water interface, and its control effect and mechanism were evaluated. The results showed that the phosphorus adsorption effect of lanthanum-modified fly ash was 34% and 40% higher compared with those of acid-modified and alkali-modified fly ash, respectively, with the phosphorus adsorption effect reaching 85%. The best dosing ratio was about 0.3 g/L. Adsorption was affected by pH and was more effective under weak alkalinity, close to the Langmuir adsorption model, which was consistent with the unimolecular layer adsorption characteristics and the presence of chemisorption and physical adsorption. The saturation adsorption amount of phosphate by lanthanum-modified fly ash was 8.89 mg/g. The optimized granulation conditions for lanthanum-modified fly ash pellets were a fly ash/montmorillonite ratio of 7:3, a roasting temperature of 900 °C, a roasting time of 4 h, and a particle size of 3 mm. After 20 days, the orthophosphate removal rate was more than 60% higher than that of the control group, with a total phosphorus removal rate of 43%. After covering for 60 days, active phosphorus in the surface layer of the sediment was gradually transformed into a stable phosphorus form, with calcium phosphorus accounting for 70% of the total inorganic phosphorus. The ability of the sediment to release phosphorus to the overlying water body was also significantly weakened. Meanwhile, the total phosphorus removal rate in the overlying water at the sediment–water interface reached more than 40%, and orthophosphate removal reached more than 60%, indicating an obvious phosphorus control effect. Transmission electron microscopy analysis showed that lanthanum was present at locations enriched with elemental phosphorus and was adsorbed onto the material surface. Therefore, lanthanum-modified fly ash pellets are a promising in situ phosphorus control agent with good endogenous phosphorus pollution control abilities in eutrophic water bodies.

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Section: Study Of Lanthanum Modified Fly Ash Pellets To Control Endog...mentioning

confidence: 99%

Control of Endogenous Phosphorus Release at the Sediment–Water Interface by Lanthanum-Modified Fly Ash

Pan

Liu²,

Chai

et al. 2022

Coatings

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Immobilization of Phosphorus in Sediment-Water System by Active Capping Plate Under Exogenous Phosphorus Input

Wu,

Lin,

Tang

et al. 2024

Water Air Soil Pollut

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Three kinds of active thin-layer capping materials for reducing the phosphorus load in eutrophic water body: comparison in dynamic experiment

Wang

Liu

et al. 2021

Environ Sci Pollut Res

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The effect of secondary capping on the control of phosphorus release from sediment by activated thin-layer capping with Al-PIA

Cited by 8 publications

References 49 publications

Control of Endogenous Phosphorus Release at the Sediment–Water Interface by Lanthanum-Modified Fly Ash

Control of Endogenous Phosphorus Release at the Sediment–Water Interface by Lanthanum-Modified Fly Ash

Immobilization of Phosphorus in Sediment-Water System by Active Capping Plate Under Exogenous Phosphorus Input

Three kinds of active thin-layer capping materials for reducing the phosphorus load in eutrophic water body: comparison in dynamic experiment

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