The important factors in sensors are sensitivity, selectivity, and response time. Oxide semiconductors are high sensitivity, fast response and the advantage of miniaturization. Zn-doped SnO 2 materials have been synthesized in order to improve the selectivity of the sensor. ZnO/ SnO 2 crystals were prepared by a simple hydrothermal process and ultrasound pretreated hydrothermal process. ZnO Received : Oct. 12, 2012, Revised : Nov. 9, 2012, Accepted : Nov. 19, 2012 This is an Open Access article distributed under the terms of the Creative Commons Attribution Non-Commercial License(http://creativecommons.org/licenses/bync/3.0)which permits unrestricted non-commercial use, distribution, and reproduction in any medium, provided the original work is properly cited.