Abstract. The terrestrial biosphere and atmospheric chemistry interact
through multiple feedbacks, but the models of vegetation and chemistry are
developed separately. In this study, the Yale Interactive terrestrial
Biosphere (YIBs) model, a dynamic vegetation model with biogeochemical
processes, is implemented into the Chemical Transport Model GEOS-Chem (GC)
version 12.0.0. Within this GC-YIBs framework, leaf area index (LAI) and
canopy stomatal conductance dynamically predicted by YIBs are used for dry
deposition calculation in GEOS-Chem. In turn, the simulated surface ozone
(O3) by GEOS-Chem affect plant photosynthesis and biophysics in YIBs.
The updated stomatal conductance and LAI improve the simulated O3 dry
deposition velocity and its temporal variability for major tree species. For
daytime dry deposition velocities, the model-to-observation correlation
increases from 0.69 to 0.76, while the normalized mean error (NME) decreases
from 30.5 % to 26.9 % using the GC-YIBs model. For the diurnal cycle, the
NMEs decrease by 9.1 % for Amazon forests, 6.8 % for coniferous forests,
and 7.9 % for deciduous forests using the GC-YIBs model. Furthermore, we
quantify the damaging effects of O3 on vegetation and find a global reduction of
annual gross primary productivity by 1.5 %–3.6 %, with regional extremes of
10.9 %–14.1 % in the eastern USA and eastern China. The online GC-YIBs
model provides a useful tool for discerning the complex feedbacks between
atmospheric chemistry and the terrestrial biosphere under global change.