2019
DOI: 10.1103/physrevlett.122.237401
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Terahertz Vortex Beam as a Spectroscopic Probe of Magnetic Excitations

Abstract: Circularly polarized light with spin angular momentum is one of the most valuable probes of magnetism. We demonstrate that light beams with orbital angular momentum (OAM), or vortex beams, can also couple to magnetism exhibiting dichroisms in a magnetized medium. Resonant optical absorption in a ferrimagnetic crystal depends strongly on both the handedness of the vortex and the direction of the beam propagation with respect to the sample magnetization. This effect exceeds the conventional dichroism for circula… Show more

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Cited by 71 publications
(51 citation statements)
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“…The standard magnetic circular dichroism with circularlypolarized light in a transmission mode in ferro-(ferri)magnets corresponds to the angularmomentum-sign dependence in the specimen constituent with M [44]. This angular-momentumsign dependence has been also observed for THz vortex beam with orbital angular momentum propagating in the film of ferrimagnetic Tb3Fe5O12 garnet [43]. Note that ferro-rotation, which does not break space inversion, does not induce optical activity, but the ferro-rotation with external electric fields has SOS with a structural chirality, and thus induces reciprocal optical activity that is linearly proportional to external electric fieldsthe so-called linear electro-gyration [45].…”
Section: Nonreciprocity With Angular Momentummentioning
confidence: 63%
See 1 more Smart Citation
“…The standard magnetic circular dichroism with circularlypolarized light in a transmission mode in ferro-(ferri)magnets corresponds to the angularmomentum-sign dependence in the specimen constituent with M [44]. This angular-momentumsign dependence has been also observed for THz vortex beam with orbital angular momentum propagating in the film of ferrimagnetic Tb3Fe5O12 garnet [43]. Note that ferro-rotation, which does not break space inversion, does not induce optical activity, but the ferro-rotation with external electric fields has SOS with a structural chirality, and thus induces reciprocal optical activity that is linearly proportional to external electric fieldsthe so-called linear electro-gyration [45].…”
Section: Nonreciprocity With Angular Momentummentioning
confidence: 63%
“…In terms of symmetry, there is no difference between spin angular momentum and orbital angular momentum. The nonreciprocity of a vortex light beam with orbital angular momentum has been, for the first time, observed for THz vortex beam propagating in ferrimagnetic Tb3Fe5O12 garnet [43]. The motion of an object with angular momentum along one direction can be linked with that in the opposite direction through {R,IM,T}, and M has broken {R,IM,T}, so M can induce nonreciprocal effect with angular momentum.…”
Section: Nonreciprocity With Angular Momentummentioning
confidence: 93%
“…Also, although there is an emerging understanding of the IFE coupling of the SAM of a beam to the electron spin, a similar understanding of the interaction of OAM with spin or orbital magnetism has still to be established. Recently, a first observation of interaction of magnetism and an OAM vortex beam in the THz regime was reported [244]. It can already be perceived that taking both spin and orbital degrees of freedom of photonic beams into account will become paramount for the future development of magnetophotonics.…”
Section: Opto-magnetism: Towards An Ultrafast Control Of Magnetismentioning
confidence: 99%
“…in order to estimate the relaxation-time dependence of the (Color online) Schematic figure of the magnon dispersion for the 3D model in Eq (30)…”
mentioning
confidence: 99%