Target Analysis Resolves the Ground and Excited State Properties from Femtosecond Stimulated Raman Spectra
Ivo H.M. van Stokkum,
Joris J. Snellenburg,
Petra Chrupková
et al.
Abstract:Target analysis is employed to resolve the ground and
excited state
properties from simultaneously measured Femtosecond Stimulated Raman
Spectra (FSRS) and Transient Absorption Spectra (TAS). FSRS is a three-pulse
technique, involving picosecond Raman pump pulses and femtosecond
visible pump and probe pulses. The TAS are needed to precisely estimate
the properties of the Instrument Response Function. The prezero “coherent
artifact” present during the overlap of the three pulses is
described by a damped oscilla… Show more
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