2022
DOI: 10.1021/acssuschemeng.2c03740
|View full text |Cite
|
Sign up to set email alerts
|

Tailoring the Properties of Self-Assembled Carbonic Anhydrase Supraparticles for CO2 Capture

Abstract: Carbon dioxide capture, conversion, and utilization with carbonic anhydrase (CA) as a green and sustainable method still faces the challenges of complex and costly purification, relatively low yield, and poor catalytic performances and reusability. Herein, we proposed an all-in-one strategy to solve these problems by self-assembling nanosized CA oligomeric particles (nCAOPs) into micrometer-sized CA supraparticles (mCASPs) with well-designed tags. The preparation of the purified mCASPs was simple and effective… Show more

Help me understand this report

Search citation statements

Order By: Relevance

Paper Sections

Select...
2
1
1
1

Citation Types

1
4
0

Year Published

2023
2023
2024
2024

Publication Types

Select...
7

Relationship

1
6

Authors

Journals

citations
Cited by 8 publications
(5 citation statements)
references
References 51 publications
(85 reference statements)
1
4
0
Order By: Relevance
“…Considering the simple purification process, high purity, and low cost of DvCA8.0-F, it will have great potentials for large-scale preparation. By staining on the micron-scale DvCA8.0-F with crystal violet, rod-shaped and ellipsoidal morphologies (Figure S4d) with sizes of about 1–2 μm were detected under an optical microscope, which was similar to some previous studies. , The formation of micron-sized supramolecules may be attributed to the complex internal and external forces, such as the hydrophobic or hydrophilic interactions, as well as electrostatic interactions between DvCA8.0 and ferritin subunits. , Additionally, high protein concentration in the cells also increases the risk of protein–protein interactions and aggregation …”
Section: Resultssupporting
confidence: 83%
See 2 more Smart Citations
“…Considering the simple purification process, high purity, and low cost of DvCA8.0-F, it will have great potentials for large-scale preparation. By staining on the micron-scale DvCA8.0-F with crystal violet, rod-shaped and ellipsoidal morphologies (Figure S4d) with sizes of about 1–2 μm were detected under an optical microscope, which was similar to some previous studies. , The formation of micron-sized supramolecules may be attributed to the complex internal and external forces, such as the hydrophobic or hydrophilic interactions, as well as electrostatic interactions between DvCA8.0 and ferritin subunits. , Additionally, high protein concentration in the cells also increases the risk of protein–protein interactions and aggregation …”
Section: Resultssupporting
confidence: 83%
“…Finally, the DvCA8.0-F with 95% purity (Figure 1b) was obtained with a yield of 800 mg/L. According to cost of the medium 57 based on a laboratory scale, it required a mere ¥22.7 (about $3.1) for the production of 1 g of DvCA8.0-F. Considering the simple purification process, high purity, and low cost of DvCA8.0-F, it will have great potentials for large-scale preparation.…”
Section: Optimization Of Co 2 Absorption and Desorption Conditionsmentioning
confidence: 99%
See 1 more Smart Citation
“…The development of catalytic SPs is a promising strategy for enhanced CO 2 reduction ability of materials. Liu et al [120] recently developed SPs with tailored properties of self-assembled carbonic anhydrase SPs for CO 2 capture. They developed SPs with simple purification and immobilization method with high yield, and excellent enzymatic properties of mCASPs and nCAOPs for sustainable CO 2 capture.…”
Section: Co 2 Reduction Applicationsmentioning
confidence: 99%
“…by using chemical or physical methods (Li et al, 2016;Fu et al, 2022). It mainly includes adsorption, lowtemperature distillation, membrane, biomimetic, physical, and chemical absorption technology (Davy, 2009;McGurk et al, 2017;Yousef et al, 2017;Luis Míguez et al, 2018;Liu et al, 2022). Among these methods, the chemical absorption is applied widely in industries because of its large absorption capacity, fast absorption rate (Shakerian et al, 2015), ability to handle large amounts of gas, and applicability to low CO 2 partial pressure gases (Muchan et al, 2022).…”
Section: Introductionmentioning
confidence: 99%