Synthetic approaches for perovskite thin films and single-crystals

Soultati, Anastasia; Tountas, Marinos; Armadorou, Konstantina‐Kalliopi; Yusoff, Abd. Rashid bin Mohd; Vasilopoulou, Maria; Nazeeruddin, Mohammad Khaja

doi:10.1039/d3ya00098b

Cited by 4 publications

(2 citation statements)

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“…On the other hand, vacuum deposition methods involve synthesizing MHPs through coevaporation under high vacuum conditions. Vacuum deposition methods can be further categorized into thermal evaporation, pulsed laser deposition, and chemical vapor deposition, whereas the colloidal nanocrystal can be synthesized by hot-injection and ligand-assisted reprecipitation. − …”

Section: Halide Perovskitesmentioning

confidence: 99%

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Halide Perovskites for Photoelectrochemical Water Splitting and CO₂ Reduction: Challenges and Opportunities

Bienkowski,

Solarska,

Trinh

et al. 2024

ACS Catal.

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Photoelectrochemical water splitting and CO2 reduction provide an attractive route to produce solar fuels while reducing the level of CO2 emissions. Metal halide perovskites (MHPs) have been extensively studied for this purpose in recent years due to their suitable optoelectronic properties. In this review, we survey the recent achievements in the field. After a brief introduction to photoelectrochemical (PEC) processes, we discussed the properties, synthesis, and application of MHPs in this context. We also survey the state-of-the-art findings regarding significant achievements in performance, and developments in addressing the major challenges of toxicity and instability toward water. Efforts have been made to replace the toxic Pb with less toxic materials like Sn, Ge, Sb, and Bi. The stability toward water has been also improved by using various methods such as compositional engineering, 2D/3D perovskite structures, surface passivation, the use of protective layers, and encapsulation. In the last part, considering the experience gained in photovoltaic applications, we provided our perspective for the future challenges and opportunities. We place special emphasis on the improvement of stability as the major challenge and the potential contribution of machine learning to identify the most suitable formulation for halide perovskites with desired properties.

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Section: Halide Perovskitesmentioning

confidence: 99%

“…Vacuum deposition methods can be further categorized into thermal evaporation, pulsed laser deposition, and chemical vapor deposition, whereas the colloidal nanocrystal can be synthesized by hot-injection and ligand-assisted reprecipitation. 114 − 116 …”

Section: Halide Perovskitesmentioning

confidence: 99%

Halide Perovskites for Photoelectrochemical Water Splitting and CO₂ Reduction: Challenges and Opportunities

Bienkowski,

Solarska,

Trinh

et al. 2024

ACS Catal.

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Strain Engineering in Perovskites: Mutual Insight on Oxides and Halides

Choi,

Lee,

Jang

2023

Advanced Materials

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Perovskite materials have garnered significant attention over the past decades due to their applications, not only in electronic materials, such as dielectrics, piezoelectrics, ferroelectrics, and superconductors but also in optoelectronic devices like solar cells and light emitting diodes. This interest arises from their versatile combinations and physiochemical tunability. While strain engineering is a recognized powerful tool for tailoring material properties, its collaborative impact on both oxides and halides remains understudied. Herein, strain engineering in perovskites for energy conversion devices, providing mutual insight into both oxides and halides is discussed. The various experimental methods are presented for applying strain by using thermal mismatch, lattice mismatch, defects, doping, light illumination, and flexible substrates. In addition, the main factors that are influenced by strain, categorized as structure (e.g., symmetry breaking, octahedral distortion), bandgap, chemical reactivity, and defect formation energy are described. After that, recent progress in strain engineering for perovskite oxides and halides for energy conversion devices is introduced. Promising methods for enhancing the performance of energy conversion devices using perovskites through strain engineering are suggested.

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The influence of the filler addition of rice husk cellulose, polyvinyl alcohol, and zinc oxide on the characteristics of environmentally friendly cassava biodegradable plastic

Hendrawati,

Liandi,

Ahyar

et al. 2023

Case Studies in Chemical and Environmental Engineering

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Synthetic approaches for perovskite thin films and single-crystals

Abstract: Halide perovskites are a compelling candidate for the next generation of clean-energy-harvesting photovoltaic technologies owing to an unprecedented increase in power conversion efficiency, their low cost, facile fabrication and outstanding...

Cited by 4 publications

References 348 publications

Halide Perovskites for Photoelectrochemical Water Splitting and CO₂ Reduction: Challenges and Opportunities

Halide Perovskites for Photoelectrochemical Water Splitting and CO₂ Reduction: Challenges and Opportunities

Strain Engineering in Perovskites: Mutual Insight on Oxides and Halides

The influence of the filler addition of rice husk cellulose, polyvinyl alcohol, and zinc oxide on the characteristics of environmentally friendly cassava biodegradable plastic

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Synthetic approaches for perovskite thin films and single-crystals

Abstract: Halide perovskites are a compelling candidate for the next generation of clean-energy-harvesting photovoltaic technologies owing to an unprecedented increase in power conversion efficiency, their low cost, facile fabrication and outstanding...

Cited by 4 publications

References 348 publications

Halide Perovskites for Photoelectrochemical Water Splitting and CO2 Reduction: Challenges and Opportunities

Halide Perovskites for Photoelectrochemical Water Splitting and CO2 Reduction: Challenges and Opportunities

Strain Engineering in Perovskites: Mutual Insight on Oxides and Halides

The influence of the filler addition of rice husk cellulose, polyvinyl alcohol, and zinc oxide on the characteristics of environmentally friendly cassava biodegradable plastic

Contact Info

Product

Resources

About

Halide Perovskites for Photoelectrochemical Water Splitting and CO₂ Reduction: Challenges and Opportunities

Halide Perovskites for Photoelectrochemical Water Splitting and CO₂ Reduction: Challenges and Opportunities