Inorganica Chimica Acta

2004

DOI: 10.1016/j.ica.2004.05.008

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Synthesis, structure and reactivity of complexes containing [M(S2)2] fragments (M=Ru, Os; (S2)2−=1,2-benzenedithiolate (2−))

Dieter Sellmann¹,

Frank W. Heinemann³

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Cited by 5 publications

References 34 publications

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Tris(dithiolene) Chemistry: A Golden Jubilee

2014

Progress in Inorganic Chemistry

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Tris(dithiolene) Chemistry: A Golden Jubilee

2014

Progress in Inorganic Chemistry

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Electronic Structure of Thiolate‐bridged Diiron Complexes and a Single‐electron Oxidation Reaction: A Combination of Experimental and Computational Studies

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³

et al. 2016

Chin. J. Chem.

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Single‐electron oxidation of a diiron‐sulfur complex [Cp*Fe(μ‐bdt)FeCp*] (1, Cp*=η5‐C5Me5; bdt=benzene‐1,2‐dithiolate) to [Cp*Fe(μ‐bdt)FeCp*]+ (2) has been experimentally conducted. The bdt ligand with redox‐active character has been computationally proposed to be a dianion (bdt2−) rather than previously proposed monoanion (bdt·−) radical in 1 though it has un‐equidistant aromatic CC bond lengths. The ground state of 1 is predicted to be two low‐spin ferrous ions (SFe=0) and 2 has a medium‐spin ferric ion (SFe=1/2) and a low‐spin ferrous center (SFe=0), and the oxidation of 1 to 2 is calculated to be a single‐metal‐based process. Both complexes have no significant antiferromagnetic coupling character.

Spin-state-dependent oxygen sensitivity of iron dithiolates: sulfur oxygenation or disulfide formation

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et al. 2008

J Biol Inorg Chem

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