“…[1][2][3] Considering their mode of charge-storage mechanisms, supercapacitors are generally categorized into two main types: (1) electrical double-layer capacitors (EDLCs), which store energy through the accumulated charge at the interface between an electrode and electrolyte; [4][5][6] (2) redox electrochemical capacitors or pseudocapacitors, where capacitance comes from reversible Faradaic reactions. [7][8][9] Presently carbonaceous materials are commonly investigated nanomaterials used in EDLCs, such as activated carbon, [10] carbon nanotubes, [11] carbon aerogels [12] and hybrid carbon. [6] As a rising star, graphene, a two-dimensional single-layer sheet of sp2-hybridized conjugated carbon atoms, has become the subject of intensive investigation in various research fields, such as energy storage, [13] solar cells, [14] and electrochemical sensors, [15][16][17] due to its excellent intrinsic electrical conductivity, extremely large specific surface area, extraordinarily superior chemical, environmental and mechanical stability.…”