“…In the work reported in this article, we used the reaction between 2,4‐toluenediisocyanate (TDI) and hydroxyl groups as the crosslinking reaction to prepare a new crosslinkable NLO polymer with side‐chains 15, 16. Both uncrosslinked copolymers, composed of methyl methacrylate (MMA), 2‐hydroxyethyl methacrylate (HEMA) and NLO chromophores, and the corresponding crosslinked systems were prepared, characterized and discussed.…”