Synthesis of Hierarchical Mesoporous ZIF-8 Functionalized with 1,2,4-Triazole by Mixed-Ligand Strategy for Enhanced CO2 Fixation Under Atmospheric Pressure
Que Thi Nguyen,
Yejin Bae,
Xuan Huy Do
et al.
Abstract:This work demonstrates the development of a hierarchical mesoporous hybrid ZIF-8 with 1,2,4-triazole (T), ZIF-8T, as a heterogeneous catalyst for CO 2 cycloaddition to epoxides under a solvent-and cocatalyst-free conditions at ambient pressure. The hybrid ZIF-8T catalyst was prepared via a facile one-pot synthesis method using a mixed-ligand of 2-methyl imidazole (2-Mim) and T. The contents of the introduced T ligand in ZIF-8T were controlled by adjusting a molar ratio of T: 2-Mim ligand. Interestingly, the ZI… Show more
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