Synthesis of CxNy-rich polycyclic oligomers from primeval monomers in aqueous media

Lavado, Nieves; Concepción, Juan García de la; Cintas, Pedro; Babiano, Reyes

doi:10.1039/d1cp05204g

Phys. Chem. Chem. Phys.

2022

DOI: 10.1039/d1cp05204g

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Synthesis of C_xN_y-rich polycyclic oligomers from primeval monomers in aqueous media

Nieves Lavado

Juan García de la Concepción

Pedro Cintas

et al.

Abstract: A multichannel, non-thermolytic and efficient pathway is described toward the formation of functionalized carbon nitride-like oligomers, starting from readily available cyanamide and glyoxal (in ratios >2), in aqueous media and...

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Novel Graphitic Oxynitrides as Photocatalysts for Sustainable H₂ Production and CO₂ Valorization. The Importance of Self‐Assembly for Catalytic Activity

Lavado,

Pardo‐Botello,

María Sánchez‐Rodas

et al. 2024

ChemSusChem

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The field of carbocatalysis, often portrayed by paradigmatic graphitic carbonaceous structures, has become a booming topic tailored for multiple applications. To this end, a new metal‐free carbocatalyst has been constructed from simple prebiotic monomers such as cyanamide and glyoxal. The resulting material shows an excellent performance as photocatalyst for H2 production and CO2 valorization, thus unveiling its real value to tackle sustainable goals. The unique oxygen‐rich carbonaceous structure has been characterized in detail, which is consistent with a graphitic layered network. The described performance in two major societal concerns along with a facile preparation from C1/C2 platforms, makes this type of overlooked oxynitride carbocatalysts promising for real‐life environmental endeavors.

show abstract

Novel Graphitic Oxynitrides as Photocatalysts for Sustainable H₂ Production and CO₂ Valorization. The Importance of Self‐Assembly for Catalytic Activity

Lavado,

Pardo‐Botello,

María Sánchez‐Rodas

et al. 2024

ChemSusChem

View full text Add to dashboard Cite

show abstract

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Synthesis of C_xN_y-rich polycyclic oligomers from primeval monomers in aqueous media

Abstract: A multichannel, non-thermolytic and efficient pathway is described toward the formation of functionalized carbon nitride-like oligomers, starting from readily available cyanamide and glyoxal (in ratios >2), in aqueous media and...

Cited by 1 publication

References 92 publications

Novel Graphitic Oxynitrides as Photocatalysts for Sustainable H₂ Production and CO₂ Valorization. The Importance of Self‐Assembly for Catalytic Activity

Novel Graphitic Oxynitrides as Photocatalysts for Sustainable H₂ Production and CO₂ Valorization. The Importance of Self‐Assembly for Catalytic Activity

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Synthesis of CxNy-rich polycyclic oligomers from primeval monomers in aqueous media

Abstract: A multichannel, non-thermolytic and efficient pathway is described toward the formation of functionalized carbon nitride-like oligomers, starting from readily available cyanamide and glyoxal (in ratios >2), in aqueous media and...

Cited by 1 publication

References 92 publications

Novel Graphitic Oxynitrides as Photocatalysts for Sustainable H2 Production and CO2 Valorization. The Importance of Self‐Assembly for Catalytic Activity

Novel Graphitic Oxynitrides as Photocatalysts for Sustainable H2 Production and CO2 Valorization. The Importance of Self‐Assembly for Catalytic Activity

Contact Info

Product

Resources

About

Synthesis of C_xN_y-rich polycyclic oligomers from primeval monomers in aqueous media

Novel Graphitic Oxynitrides as Photocatalysts for Sustainable H₂ Production and CO₂ Valorization. The Importance of Self‐Assembly for Catalytic Activity

Novel Graphitic Oxynitrides as Photocatalysts for Sustainable H₂ Production and CO₂ Valorization. The Importance of Self‐Assembly for Catalytic Activity