Synthesis of ABCBA-type miktoarm H-shaped copolymers with poly(3-hexylthiophene) segments and their application to intrinsically stretchable photonic transistor memory

Inagaki, Shin; Sung, Chih‐Yuan; Chang, Ai‐Chun; Lin, Yan‐Cheng; Chen, Wen‐Chang; Higashihara, Tomoya

doi:10.1039/d3tc00690e

J. Mater. Chem. C

2023

DOI: 10.1039/d3tc00690e

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Synthesis of ABCBA-type miktoarm H-shaped copolymers with poly(3-hexylthiophene) segments and their application to intrinsically stretchable photonic transistor memory

Shin Inagaki

Chih‐Yuan Sung

Ai‐Chun Chang

et al.

Abstract: Recently, semiconducting polymers with intrinsic elasticity have garnered attention for their application in wearable devices. Herein, we synthesized a novel ABCBA-type miktoarm H-shaped copolymer (where A, B, and C represent...

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Intrinsically Stretchable and Healable Polymer Semiconductors

Xue,

Li,

Shangguan

et al. 2023

Advanced Science

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In recent decades, polymer semiconductors, extensively employed as charge transport layers in devices like organic field‐effect transistors (OFETs), have undergone thorough investigation due to their capacity for large‐area solution processing, making them promising for mass production. Research efforts have been twofold: enhancing the charge mobilities of polymer semiconductors and augmenting their mechanical properties to meet the demands of flexible devices. Significant progress has been made in both realms, propelling the practical application of polymer semiconductors in flexible electronics. However, integrating excellent semiconducting and mechanical properties into a single polymer still remains a significant challenge. This review intends to introduce the design strategies and discuss the properties of high‐charge mobility stretchable conjugated polymers. In addition, another key challenge faced in this cutting‐edge field is maintaining stable semiconducting performance during long‐term mechanical deformations. Therefore, this review also discusses the development of healable polymer semiconductors as a promising avenue to improve the lifetime of stretchable device. In conclusion, challenges and outline future research perspectives in this interdisciplinary field are highlighted.

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Intrinsically Stretchable and Healable Polymer Semiconductors

Xue,

Li,

Shangguan

et al. 2023

Advanced Science

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Enhanced performance of phototransistor memory by optimizing the block copolymer architectures comprising Polyfluorenes and hydrogen-bonded insulating coils

Lin,

Wu,

Hsieh

et al. 2024

Polymer

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Boosting the charge injection of polymer electrets for light-stimulated artificial synaptic transistors

Li,

Hu,

Zhu

et al. 2024

J. Mater. Chem. C

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Synthesis of ABCBA-type miktoarm H-shaped copolymers with poly(3-hexylthiophene) segments and their application to intrinsically stretchable photonic transistor memory

Abstract: Recently, semiconducting polymers with intrinsic elasticity have garnered attention for their application in wearable devices. Herein, we synthesized a novel ABCBA-type miktoarm H-shaped copolymer (where A, B, and C represent...

Cited by 3 publications

References 52 publications

Intrinsically Stretchable and Healable Polymer Semiconductors

Intrinsically Stretchable and Healable Polymer Semiconductors

Enhanced performance of phototransistor memory by optimizing the block copolymer architectures comprising Polyfluorenes and hydrogen-bonded insulating coils

Boosting the charge injection of polymer electrets for light-stimulated artificial synaptic transistors

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