Abstract:Satellite‐ and ground‐based remote sensing are two widely used techniques to measure aerosol properties. However, neither is perfect in that satellite retrievals suffer from various sources of uncertainties, and ground observations have limited spatial coverage. In this study, focusing on improving estimates of aerosol information on large scale, we develop a data synergy technique based on the ensemble Kalman filter (EnKF) to effectively combine these two types of measurements and yield a monthly mean aerosol… Show more
“…erefore, the research on management of PM2.5 and PM10 has become a hot topic in recent years. Besides, it is found to significantly affect the cloud formation and precipitation through aerosol-radiation interaction or aerosol-cloud interaction [10][11][12][13][14], even though the net effect remains highly debated [15][16][17]. e main factors affecting the concentration of atmospheric particulate matter include emission sources and meteorological factors [18][19][20][21][22][23][24].…”
In this paper, hourly observations of precipitation, wind, and PM2.5 and PM10 concentrations in Qinhuangdao from 2016 to 2018 were used to study the effects of precipitation and wind on PM2.5 and PM10 concentrations. The results show that precipitation has a certain wet scavenging effect on PM2.5 and PM10, and the scavenging effect on PM10 is greater than that on PM2.5. Precipitation above moderate rainfall is concentrated from May to September, and light rain in winter increases the concentration of pollutants. The changes of PM2.5 before and after precipitation are related to the initial concentration of PM2.5 before precipitation, precipitation intensity, and precipitation duration. The scavenging effect of precipitation on PM10 is closely related to the initial concentration of PM10 before precipitation. The higher the initial concentration of PM10 is, the greater the removal amount of precipitation will be. Moderate or above pollution weather mainly occurs in the northeast, southwest, and west wind meteorological conditions; the more westerly the wind, the more the pollution; north wind and northwest wind have the most obvious scavenging effect on PM2.5 and Pm10; when the wind speed increases to 2 m/s, the concentration of PM2.5 and PM10 can be reduced; when the wind speed is more than 4 m/s, the concentration of PM10 increases under the south wind, southeast wind, east wind, and northeast wind.
“…erefore, the research on management of PM2.5 and PM10 has become a hot topic in recent years. Besides, it is found to significantly affect the cloud formation and precipitation through aerosol-radiation interaction or aerosol-cloud interaction [10][11][12][13][14], even though the net effect remains highly debated [15][16][17]. e main factors affecting the concentration of atmospheric particulate matter include emission sources and meteorological factors [18][19][20][21][22][23][24].…”
In this paper, hourly observations of precipitation, wind, and PM2.5 and PM10 concentrations in Qinhuangdao from 2016 to 2018 were used to study the effects of precipitation and wind on PM2.5 and PM10 concentrations. The results show that precipitation has a certain wet scavenging effect on PM2.5 and PM10, and the scavenging effect on PM10 is greater than that on PM2.5. Precipitation above moderate rainfall is concentrated from May to September, and light rain in winter increases the concentration of pollutants. The changes of PM2.5 before and after precipitation are related to the initial concentration of PM2.5 before precipitation, precipitation intensity, and precipitation duration. The scavenging effect of precipitation on PM10 is closely related to the initial concentration of PM10 before precipitation. The higher the initial concentration of PM10 is, the greater the removal amount of precipitation will be. Moderate or above pollution weather mainly occurs in the northeast, southwest, and west wind meteorological conditions; the more westerly the wind, the more the pollution; north wind and northwest wind have the most obvious scavenging effect on PM2.5 and Pm10; when the wind speed increases to 2 m/s, the concentration of PM2.5 and PM10 can be reduced; when the wind speed is more than 4 m/s, the concentration of PM10 increases under the south wind, southeast wind, east wind, and northeast wind.
“…This quantity is widely used as a constraint on climate models or for model evaluation (e.g., Buchard et al, 2017;Gelaro et al, 2017;Gliß et al, 2021;Kinne et al, 2006;Randles et al, 2017;Rubin et al, 2017;Schutgens et al, 2020), though non-negligible differences among AOD retrieval products must yet be addressed (J. Li et al, 2020;Sogacheva et al, 2020). Tables summarizing currently available satellite AOD products are given in Sogacheva et al (2020) and Kahn and Samset (2022).…”
Section: Aerosol Amount-total-column Optical Depth and 3-d Distributionmentioning
Aerosol forcing uncertainty represents the largest climate forcing uncertainty overall. Its magnitude has remained virtually undiminished over the past 20 years despite considerable advances in understanding most of the key contributing elements. Recent work has produced modest increases only in the confidence of the uncertainty estimate itself. This review summarizes the contributions toward reducing the uncertainty in the aerosol forcing of climate made by satellite observations, measurements taken within the atmosphere, as well as modeling and data assimilation. We adopt a more measurement‐oriented perspective than most reviews of the subject in assessing the strengths and limitations of each; gaps and possible ways to fill them are considered. Currently planned programs supporting advanced, global‐scale satellite and surface‐based aerosol, cloud, and precursor gas observations, climate modeling, and intensive field campaigns aimed at characterizing the underlying physical and chemical processes involved, are all essential. But in addition, new efforts are needed: (a) to obtain systematic aircraft in situ measurements capturing the multi‐variate probability distribution functions of particle optical, microphysical, and chemical properties (and associated uncertainty estimates), as well as co‐variability with meteorology, for the major aerosol airmass types; (b) to conceive, develop, and implement a suborbital (aircraft plus surface‐based) program aimed at systematically quantifying the cloud‐scale microphysics, cloud optical properties, and cloud‐related vertical velocities associated with aerosol‐cloud interactions; and (c) to focus much more research on integrating the unique contributions of satellite observations, suborbital measurements, and modeling, to reduce the persistent uncertainty in aerosol climate forcing.
“…In-situ observations of aerosol and cloud interaction are essential for improving our fundamental understanding of their role in the climate system [59]. Properties of aerosolcloud interactions in the climate change Arctic hotspot are an important input to climate models, while the impact of clouds remains one of the largest uncertainties [60,61]. The 7th Pallas Cloud Experiment (PaCE) in Finland was organized in September 2017 and focused on cloud-aerosol interactions through in-situ and remote sensing methods.…”
Section: Profiling Of Aerosol-cloud Interaction Observations Over Northern Finlandmentioning
The Unmanned Systems Research Laboratory (USRL) of the Cyprus Institute is a new mobile exploratory platform of the EU Research Infrastructure Aerosol, Clouds and Trace Gases Research InfraStructure (ACTRIS). USRL offers exclusive Unmanned Aerial Vehicle (UAV)-sensor solutions that can be deployed anywhere in Europe and beyond, e.g., during intensive field campaigns through a transnational access scheme in compliance with the drone regulation set by the European Union Aviation Safety Agency (EASA) for the research, innovation, and training. UAV sensor systems play a growing role in the portfolio of Earth observation systems. They can provide cost-effective, spatial in-situ atmospheric observations which are complementary to stationary observation networks. They also have strong potential for calibrating and validating remote-sensing sensors and retrieval algorithms, mapping close-to-the-ground emission point sources and dispersion plumes, and evaluating the performance of atmospheric models. They can provide unique information relevant to the short- and long-range transport of gas and aerosol pollutants, radiative forcing, cloud properties, emission factors and a variety of atmospheric parameters. Since its establishment in 2015, USRL is participating in major international research projects dedicated to (1) the better understanding of aerosol-cloud interactions, (2) the profiling of aerosol optical properties in different atmospheric environments, (3) the vertical distribution of air pollutants in and above the planetary boundary layer, (4) the validation of Aeolus satellite dust products by utilizing novel UAV-balloon-sensor systems, and (5) the chemical characterization of ship and stack emissions. A comprehensive overview of the new UAV-sensor systems developed by USRL and their field deployments is presented here. This paper aims to illustrate the strong scientific potential of UAV-borne measurements in the atmospheric sciences and the need for their integration in Earth observation networks.
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