2023
DOI: 10.1039/d2mh01495e
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Synergistic effects of extrinsic photoconduction and photogating in a short-wavelength ZrS3 infrared photodetector

Abstract: Two-dimensional (2D) material-based photodetectors, especially those working in the infrared band, have shown great application potential in thermal imaging, optical communication, and medicine fields. Designing 2D material photodetectors with broadened...

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Cited by 8 publications
(10 citation statements)
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References 49 publications
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“…For a typical photogating effect in a pure MoS 2 device, long carrier lifetimes result in substantial gains but slower response times. 44 In comparison to a pure MoS 2 device, the phototransistor based on V-doped MoS 2 exhibits a significantly improved response speed by 3 orders of magnitude, reaching 3 ms. This enhancement may be attributed to the sensitivity of the response time in atomically thin MoS 2 to the states of defects.…”
Section: Resultsmentioning
confidence: 98%
“…For a typical photogating effect in a pure MoS 2 device, long carrier lifetimes result in substantial gains but slower response times. 44 In comparison to a pure MoS 2 device, the phototransistor based on V-doped MoS 2 exhibits a significantly improved response speed by 3 orders of magnitude, reaching 3 ms. This enhancement may be attributed to the sensitivity of the response time in atomically thin MoS 2 to the states of defects.…”
Section: Resultsmentioning
confidence: 98%
“…S18, ESI†). 60,61 In addition, the dependence of the photocurrent on light power density has been fitted by the power law. Under various illuminations, the fitting factors are all far less than 1 (0.39–0.66, Fig.…”
Section: Resultsmentioning
confidence: 99%
“…The excess photogenerated electrons in GeSe may circulate several times before recombining with the holes, which leads to an enhanced photoconductive gain in the device. Recently, Yu et al have reported a similar photogating effect due to natural oxidation in ZrS 3 -based IR photodetectors . Intuitively, a capping layer of hBN or Al 2 O 3 could truncate the process of oxidation in GeSe, but the self-assembled GeO x /GeSe heterostructure imparts a broadband detection capability to the device, without jeopardizing the detection capability of the pristine GeSe layer underneath.…”
Section: Resultsmentioning
confidence: 99%
“…Recently, Yu et al have reported a similar photogating effect due to natural oxidation in ZrS 3 -based IR photodetectors. 39 Intuitively, a capping layer of hBN or Al 2 O 3 could truncate the process of oxidation in GeSe, but the self-assembled GeO x /GeSe heterostructure imparts a broadband detection capability to the device, without jeopardizing the detection capability of the pristine GeSe layer underneath. It is worth mentioning that most of the existing reports on GeSe photodetectors and phototransistors focus on eliminating or overlooking the defect states and oxidation in GeSe, and thus, little consideration has been devoted toward harnessing their inherent capabilities in optical devices.…”
mentioning
confidence: 99%